Evolution of nanodomains in 0.9PbMg1/3Nb2/3O3-0.1PbTiO3 single crystals

被引:98
作者
Shvartsman, V. V. [1 ]
Kholkin, A. L.
机构
[1] Univ Duisburg Essen, D-47048 Duisburg, Germany
[2] Univ Aveiro, Dept Ceram & Glass Engn, CICECO, P-3810193 Aveiro, Portugal
关键词
D O I
10.1063/1.2713084
中图分类号
O59 [应用物理学];
学科分类号
摘要
High-resolution studies of polar structures have been performed on the 0.9Pb(Mg1/3Nb2/3)O-3-0.1PbTiO(3) (0.9PMN-0.1PT) single crystals by piezoresponse force microscopy. A complex pattern of nanosized polar regions (nanodomains) was observed above the temperature of the structural phase transition. Autocorrelation function technique applied to the analysis of the obtained images revealed clear self-organization of the nanodomains in (110) crystallographic directions and allowed estimating their mean size (similar to 70 nm at room temperature). Upon heating, the gradual decay of the piezoresponse contrast took place, however, the nanodomains could be still observed at temperatures as high as 385 K. The nature of the observed phenomena is attributed to a peculiar transient state between relaxor and ferroelectric, which developed near the crystal's surface. (c) 2007 American Institute of Physics.
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页数:5
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