Hollow spherical nanocapsules of poly(pyrrole) as a promising support for Pt/Ru nanoparticles based catalyst

被引:16
作者
Choi, Seong-Ho [1 ]
Gopalan, Anantha Iyengar [2 ]
Ryu, Jung-Ho [1 ]
Lee, Kwang-Pill [2 ]
机构
[1] Hannam Univ, BK NanoBiosensor Res Team 21, Dept Chem, Taejon 305811, South Korea
[2] Kyungpook Natl Univ, Dept Chem, Grad Sch, Taegu 702701, South Korea
基金
新加坡国家研究基金会;
关键词
Nanostructures; Poly(pyrrole); Radiation; Catalyst support; PtRu nanoparticles; METHANOL FUEL-CELLS; GAMMA-RADIATION SYNTHESIS; WALLED CARBON NANOTUBES; PT-RU CATALYST; GOLD NANOPARTICLES; CONTROLLED GROWTH; ALLOY CATALYSTS; ELECTROCATALYSTS; SIZE; POLYANILINE;
D O I
10.1016/j.matchemphys.2009.11.035
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Poly(pyrrole) hollow spherical nanocapsules (HSNCs-PPy) were prepared and used as an efficient support matrix to PtRu nanoparticles. gamma-Radiation was utilized to load PtRu nanoparticles into Ppy-HSNC matrix. The advantageous characteristics of HSNCs-Ppy/PtRu catalyst as a support matrix for loading PtRu catalysts are presented. (C) 2009 Elsevier B.V. All rights reserved.
引用
收藏
页码:18 / 22
页数:5
相关论文
共 53 条
[1]  
AFICO AS, 2001, FUEL CELL, V1, P133
[2]   Shape-controlled synthesis of colloidal platinum nanoparticles [J].
Ahmadi, TS ;
Wang, ZL ;
Green, TC ;
Henglein, A ;
ElSayed, MA .
SCIENCE, 1996, 272 (5270) :1924-1926
[3]   Platinum-based ternary catalysts for low temperature fuel cells Part I. Preparation methods and structural characteristics [J].
Antolini, Ermete .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2007, 74 (3-4) :324-336
[4]   The stability of Pt-M (M = first row transition metal) alloy catalysts and its effect on the activity in low temperature fuel cells - A literature review and tests on a Pt-Co catalyst [J].
Antolini, Ermete ;
Salgado, Jose R. C. ;
Gonzalez, Ernesto R. .
JOURNAL OF POWER SOURCES, 2006, 160 (02) :957-968
[5]   Challenges and breakthroughs in recent research on self-assembly [J].
Ariga, Katsuhiko ;
Hill, Jonathan P. ;
Lee, Michael V. ;
Vinu, Ajayan ;
Charvet, Richard ;
Acharya, Somobrata .
SCIENCE AND TECHNOLOGY OF ADVANCED MATERIALS, 2008, 9 (01)
[6]   Microwave synthesis of polymer-embedded Pt-Ru catalyst for direct methanol fuel cell [J].
Bensebaa, F ;
Farah, AA ;
Wang, DS ;
Bock, C ;
Du, XM ;
Kung, J ;
Le Page, Y .
JOURNAL OF PHYSICAL CHEMISTRY B, 2005, 109 (32) :15339-15344
[7]   Size-selected synthesis of PtRu nano-catalysts: Reaction and size control mechanism [J].
Bock, C ;
Paquet, C ;
Couillard, M ;
Botton, GA ;
MacDougall, BR .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2004, 126 (25) :8028-8037
[8]   Study of nickel catalysts supported on silica of low surface area and prepared by reduction of nickel acetate in aqueous hydrazine [J].
Boudjahem, AG ;
Monteverdi, S ;
Mercy, M ;
Bettahar, MM .
JOURNAL OF CATALYSIS, 2004, 221 (02) :325-334
[9]   SYNTHESIS OF THIOL-DERIVATIZED GOLD NANOPARTICLES IN A 2-PHASE LIQUID-LIQUID SYSTEM [J].
BRUST, M ;
WALKER, M ;
BETHELL, D ;
SCHIFFRIN, DJ ;
WHYMAN, R .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1994, (07) :801-802
[10]   Novel nanocomposite Pt/RuO2•xH2O/carbon nanotube catalysts for direct methanol fuel cells [J].
Cao, Lin ;
Scheiba, Frieder ;
Roth, Christina ;
Schweiger, Franz ;
Cremers, Carsten ;
Stimming, Ulrich ;
Fuess, Hartmut ;
Chen, Liquan ;
Zhu, Wentao ;
Qiu, Xinping .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2006, 45 (32) :5315-5319