Time-resolved studies with FELs

被引：19

作者：

Rudenko, Artem ^{[1
,2
]}

Rolles, Daniel ^{[1
,3
]}

机构：

[1] Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA

[2] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany

[3] Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany

来源：

JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA | 2015年 / 204卷

关键词：

Ultrafast X-ray science; Pump-probe experiments; Photoelectron imaging; Coincidence momentum imaging; Free-electron lasers; FREE-ELECTRON LASER; EXTREME-ULTRAVIOLET; CHARGE-TRANSFER; OPTICAL PULSES; ULTRA-SHORT; GENERATION; MOLECULES; COHERENT; LOCALIZATION; IONIZATION;

D O I：

10.1016/j.elspec.2015.07.010

中图分类号：

O433 [光谱学];

学科分类号：

0703 ; 070302 ;

摘要：

Intense femtosecond VUV, XUV, and X-ray pulses from free-electron lasers (FELs) enable time-resolved experiments studying ultrafast dynamics in a large variety of systems relevant, e.g., to physics, chemistry, biology, and material sciences. In this paper, we focus on time-resolved studies of gas-phase molecules, which lie at the crossroad between atomic, molecular and optical physics and ultrafast photochemistry. We describe the current status of the field and discuss typical experimental configurations used for pump-probe experiments with FELs. We illustrate them with three recent examples for such experiments performed at the FLASH and LCLS FELs studying charge transfer following XUV and X-ray photoabsorption as well as photoelectron diffraction from aligned molecules. We conclude with a short outlook on future developments and perspectives for femtosecond pump-probe experiments with FELs. (C) 2015 Elsevier B.V. All rights reserved.

引用

页码：228 / 236

页数：9

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