HETEROGENEOUS CATALYSIS Confined microenvironment for catalysis control

被引:81
作者
Fu, Qiang [1 ]
Bao, Xinhe [1 ]
机构
[1] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian, Peoples R China
关键词
D O I
10.1038/s41929-019-0354-z
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The design of heterogeneous catalysts with tunable activity and selectivity constitutes a remarkable challenge. Now, a synthetic approach towards producing nanocrystals encapsulated within polymer layers has been developed, unravelling the principles to achieve control of transition state and product diffusion using CO oxidation as a case study.
引用
收藏
页码:834 / 836
页数:3
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共 9 条
  • [1] Reactions at surfaces: From atoms to complexity (Nobel lecture)
    Ertl, Gerhard
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2008, 47 (19) : 3524 - 3535
  • [2] Confined catalysis under two-dimensional materials
    Li, Haobo
    Xiao, Jianping
    Fu, Qiang
    Bao, Xinhe
    [J]. PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2017, 114 (23) : 5930 - 5934
  • [3] Confinement Effects in Catalysis Using Well-Defined Materials and Cages
    Mouarrawis, Valentinos
    Plessius, Raoul
    van der Vlugt, Jarl Ivar
    Reek, Joost N. H.
    [J]. FRONTIERS IN CHEMISTRY, 2018, 6
  • [4] The nature of the active site in heterogeneous metal catalysis
    Norskov, Jens K.
    Bligaard, Thomas
    Hvolbaek, Britt
    Abild-Pedersen, Frank
    Chorkendorff, Ib
    Christensen, Claus H.
    [J]. CHEMICAL SOCIETY REVIEWS, 2008, 37 (10) : 2163 - 2171
  • [5] Transition state and product diffusion control by polymer-nanocrystal hybrid catalysts
    Riscoe, Andrew R.
    Wrasman, Cody J.
    Herzing, Andrew A.
    Hoffman, Adam S.
    Menon, Aditya
    Boubnov, Alexey
    Vargas, Maria
    Bare, Simon R.
    Cargnello, Matteo
    [J]. NATURE CATALYSIS, 2019, 2 (10) : 852 - 863
  • [6] The confinement effect in zeolites
    Sastre, G.
    Corma, A.
    [J]. JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL, 2009, 305 (1-2) : 3 - 7
  • [7] A theory of the catalytic surface
    Taylor, HS
    [J]. PROCEEDINGS OF THE ROYAL SOCIETY OF LONDON SERIES A-CONTAINING PAPERS OF A MATHEMATICAL AND PHYSICAL CHARACTER, 1925, 108 (745) : 105 - 111
  • [8] Catalysis: principles, progress, prospects
    Thomas, JM
    Williams, JP
    [J]. PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES, 2005, 363 (1829): : 765 - 791
  • [9] Toward Fundamentals of Confined Catalysis in Carbon Nanotubes
    Xiao, Jianping
    Pan, Xiulian
    Guo, Shujing
    Ren, Pengju
    Bao, Xinhe
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2015, 137 (01) : 477 - 482