Room-Temperature Near-Infrared High-Q Perovskite Whispering-Gallery Planar Nano lasers

被引:739
作者
Zhang, Qing [1 ]
Ha, Son Tung [1 ]
Liu, Xinfeng [1 ,2 ]
Sum, Tze Chien [1 ,2 ,3 ]
Xiong, Qihua [1 ,3 ,4 ]
机构
[1] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore
[2] Nanyang Technol Univ, Energy Res Inst NTU ERI N, Singapore 637553, Singapore
[3] Singapore Berkeley Res Initiat Sustainable Energy, Singapore 138602, Singapore
[4] Nanyang Technol Univ, Sch Elect & Elect Engn, Nanoelect Ctr Excellence, NOVITAS, Singapore 639798, Singapore
基金
新加坡国家研究基金会;
关键词
Organic-inorganic perovskites; whispering gallery mode lasing; near-infrared lasers; nanoplatelets; wavelength tunable; on-chip integration; MODES; EFFICIENCY;
D O I
10.1021/nl503057g
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Near-infrared (NIR) solid state micro/nanolasers are improtant building blocks for true integration of optoelectronic circuitry.(1) Although significant progress has been made in III-V nanowire lasers with achieving NIR lasing at room temperature,(2-4) challenges remain including low quantum efficiencies and high auger losses. Imporatntly, the obstacles toward integrating one-dimensioanl nanowires on the planar ubquitous Si platform need to be effectively tackled. Here we demonstrate a new family of planar room-temperature NIR nanolasers based on organic-inorganic perovskite CH3NH3PbI3-aXa (X = I, Br, Cl) nanoplatelets. Their large exciton binding energies, long diffusion lengths, and naturally formed high quality planar whispering-gallery mode cavities ensure adequate gain and efficient optical feedback for low-threshold optically pumpbed in-plane lasing. We show that these remarkable wavelength tunable whispering-gallery nanolasers can be easily integrated onto conductive platforms (Si, Au, indium tin oxidie, and so forth). Our findings open up a new class of wavelength tunable palanar nanomaterials potentially suitable for on-chip integration.
引用
收藏
页码:5995 / 6001
页数:7
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