Revised estimates of ocean-atmosphere CO2 flux are consistent with ocean carbon inventory

被引:173
作者
Watson, Andrew J. [1 ]
Schuster, Ute [1 ]
Shutler, Jamie D. [1 ]
Holding, Thomas [1 ]
Ashton, Ian G. C. [1 ]
Landschuetzer, Peter [2 ]
Woolf, David K. [3 ]
Goddijn-Murphy, Lonneke [4 ]
机构
[1] Univ Exeter, Coll Life & Environm Sci, Exeter, Devon, England
[2] Max Planck Inst Meteorol, Bunderstr 53, D-20146 Hamburg, Germany
[3] Heriot Watt Univ, Int Ctr Isl Technol, Stromness, Orkney, England
[4] Univ Highlands & Isl, Environm Res Inst, Ormlie Rd, Thurso, Scotland
基金
英国自然环境研究理事会; 欧盟地平线“2020”;
关键词
SURFACE-OCEAN; GAS-EXCHANGE; VARIABILITY; TEMPERATURE; ATLANTIC; PCO(2); SATELLITE; SUPPORT; RECORD; BUDGET;
D O I
10.1038/s41467-020-18203-3
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
The ocean is a sink for similar to 25% of the atmospheric CO2 emitted by human activities, an amount in excess of 2 petagrams of carbon per year (PgCyr(-1)). Time-resolved estimates of global ocean-atmosphere CO2 flux provide an important constraint on the global carbon budget. However, previous estimates of this flux, derived from surface ocean CO2 concentrations, have not corrected the data for temperature gradients between the surface and sampling at a few meters depth, or for the effect of the cool ocean surface skin. Here we calculate a time history of ocean-atmosphere CO2 fluxes from 1992 to 2018, corrected for these effects. These increase the calculated net flux into the oceans by 0.8-0.9 PgC yr(-1), at times doubling uncorrected values. We estimate uncertainties using multiple interpolation methods, finding convergent results for fluxes globally after 2000, or over the Northern Hemisphere throughout the period. Our corrections reconcile surface uptake with independent estimates of the increase in ocean CO2 inventory, and suggest most ocean models underestimate uptake.
引用
收藏
页数:6
相关论文
共 40 条
[1]   A multi-decade record of high-quality fCO2 data in version 3 of the Surface Ocean CO2 Atlas (SOCAT) [J].
Bakker, Dorothee C. E. ;
Pfeil, Benjamin ;
Landa, Camilla S. ;
Metzl, Nicolas ;
O'Brien, Kevin M. ;
Olsen, Are ;
Smith, Karl ;
Cosca, Cathy ;
Harasawa, Sumiko ;
Jones, Stephen D. ;
Nakaoka, Shin-ichiro ;
Nojiri, Yukihiro ;
Schuster, Ute ;
Steinhoff, Tobias ;
Sweeney, Colm ;
Takahashi, Taro ;
Tilbrook, Bronte ;
Wada, Chisato ;
Wanninkhof, Rik ;
Alin, Simone R. ;
Balestrini, Carlos F. ;
Barbero, Leticia ;
Bates, Nicholas R. ;
Bianchi, Alejandro A. ;
Bonou, Frederic ;
Boutin, Jacqueline ;
Bozec, Yann ;
Burger, Eugene F. ;
Cai, Wei-Jun ;
Castle, Robert D. ;
Chen, Liqi ;
Chierici, Melissa ;
Currie, Kim ;
Evans, Wiley ;
Featherstone, Charles ;
Feely, Richard A. ;
Fransson, Agneta ;
Goyet, Catherine ;
Greenwood, Naomi ;
Gregor, Luke ;
Hankin, Steven ;
Hardman-Mountford, Nick J. ;
Harlay, Jerome ;
Hauck, Judith ;
Hoppema, Mario ;
Humphreys, Matthew P. ;
Hunt, ChristopherW. ;
Huss, Betty ;
Ibanhez, J. Severino P. ;
Johannessen, Truls .
EARTH SYSTEM SCIENCE DATA, 2016, 8 (02) :383-413
[2]   A long-term record of blended satellite and in situ sea-surface temperature for climate monitoring, modeling and environmental studies [J].
Banzon, Viva ;
Smith, Thomas M. ;
Chin, Toshio Mike ;
Liu, Chunying ;
Hankins, William .
EARTH SYSTEM SCIENCE DATA, 2016, 8 (01) :165-176
[3]   Reassessing Southern Ocean Air-Sea CO2 Flux Estimates With the Addition of Biogeochemical Float Observations [J].
Bushinsky, Seth M. ;
Landschuetzer, Peter ;
Roedenbeck, Christian ;
Gray, Alison R. ;
Baker, David ;
Mazloff, Matthew R. ;
Resplandy, Laure ;
Johnson, Kenneth S. ;
Sarmiento, Jorge L. .
GLOBAL BIOGEOCHEMICAL CYCLES, 2019, 33 (11) :1370-1388
[4]   Variation of PCO2 along a North Atlantic shipping route (UK to the Caribbean):: A year of automated observations [J].
Cooper, DJ ;
Watson, AJ ;
Ling, RD .
MARINE CHEMISTRY, 1998, 60 (1-2) :147-164
[5]   LSCE-FFNN-v1: a two-step neural network model for the reconstruction of surface ocean pCO2 over the global ocean [J].
Denvil-Sommer, Anna ;
Gehlen, Marion ;
Vrac, Mathieu ;
Mejia, Carlos .
GEOSCIENTIFIC MODEL DEVELOPMENT, 2019, 12 (05) :2091-2105
[6]  
Dlugokencky E.J., 2017, NOAA Greenhouse Gas Reference from Atmospheric Carbon Dioxide Dry Air Mole Fractions from the NOAA ESRL Carbon Cycle Cooperative Global Air Sampling Network
[7]  
Donlon CJ, 2002, J CLIMATE, V15, P353, DOI 10.1175/1520-0442(2002)015<0353:TIVOSS>2.0.CO
[8]  
2
[9]   Global open-ocean biomes: mean and temporal variability [J].
Fay, A. R. ;
McKinley, G. A. .
EARTH SYSTEM SCIENCE DATA, 2014, 6 (02) :273-284
[10]   The OceanFlux Greenhouse Gases methodology for deriving a sea surface climatology of CO2 fugacity in support of air-sea gas flux studies [J].
Goddijn-Murphy, L. M. ;
Woolf, D. K. ;
Land, P. E. ;
Shutler, J. D. ;
Donlon, C. .
OCEAN SCIENCE, 2015, 11 (04) :519-541