Mechanochemical Synthesis of Catalytic Materials

被引:202
作者
Amrute, Amol P. [1 ,2 ]
De Bellis, Jacopo [1 ]
Felderhoff, Michael [1 ]
Schueth, Ferdi [1 ]
机构
[1] Max Planck Inst Kohlenforsch, Dept Heterogeneous Catalysis, Kaiser Wilhelm Pl 1, D-45470 Mulheim, Germany
[2] ASTAR, Inst Chem & Engn Sci, 1 Pesek Rd, Singapore 627833, Singapore
关键词
ball milling; catalyst synthesis; comminution; heterogeneous catalysis; mechanochemistry; nanomaterials; METAL-ORGANIC FRAMEWORKS; PEROVSKITE-TYPE OXIDES; IN-SITU; REAL-TIME; MECHANOCATALYTIC DEPOLYMERIZATION; PHASE-TRANSFORMATIONS; MILLING REACTIONS; OXYGEN REDUCTION; ACTIVE CATALYST; CARBON-MONOXIDE;
D O I
10.1002/chem.202004583
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The mechanochemical synthesis of nanomaterials for catalytic applications is a growing research field due to its simplicity, scalability, and eco-friendliness. Besides, it provides materials with distinct features, such as nanocrystallinity, high defect concentration, and close interaction of the components in a system, which are, in most cases, unattainable by conventional routes. Consequently, this research field has recently become highly popular, particularly for the preparation of catalytic materials for various applications, ranging from chemical production over energy conversion catalysis to environmental protection. In this Review, recent studies on mechanochemistry for the synthesis of catalytic materials are discussed. Emphasis is placed on the straightforwardness of the mechanochemical route-in contrast to more conventional synthesis-in fabricating the materials, which otherwise often require harsh conditions. Distinct material properties achieved by mechanochemistry are related to their improved catalytic performance.
引用
收藏
页码:6819 / 6847
页数:29
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