Double-Shell and Flower-Like ZnS-C3N4 Derived from in Situ Supramolecular Self-Assembly for Selective Aerobic Oxidation of Amines to Imines

被引:46
|
作者
Chen, Peng [1 ]
Meng, Ling-Hu [1 ]
Chen, Lang [1 ]
Guo, Jun-Kang [1 ]
Shen, Sheng [1 ]
Au, Chak-Tong [2 ]
Yin, Shuang-Feng [1 ]
机构
[1] Hunan Univ, Coll Chem & Chem Engn, State Key Lab Chemo Biosensing & Chemometr, Prov Hunan Key Lab Cost Effect Utilizat Fossil Fu, Lushan South Rd, Changsha 410082, Hunan, Peoples R China
[2] Hunan Inst Engn, Coll Chem & Chem Engn, Fuxing East Rd, Xiangtan 411104, Hunan, Peoples R China
基金
中国国家自然科学基金;
关键词
Double shell; Flower-like ZnS-C3N4; Self-assembly; Selective oxidation; Photocatalysis; VISIBLE-LIGHT DRIVEN; HOLLOW MICROSPHERES; EFFICIENT; WATER; HETEROJUNCTION; PHOTOCATALYSTS; NANOSHEETS; FABRICATION; SEPARATION; COMPOSITE;
D O I
10.1021/acssuschemeng.9b02969
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Multishelled micro-/nanostructures have attracted much research attention because of their unique properties. It is a big challenge to fabricate multishelled hollow structures of complex nanoarchitectures with the respective shells different in composition. Herein, the double-shell and flower-like ZnS-C3N4 (2-ZSCN) was fabricated by a facile supramolecular self-assembly method. Because of its unique structure, 2-ZSCN exhibits enhanced photocatalytic activity and stability in the selective aerobic oxidation of amines to imines under visible-light irradiation.
引用
收藏
页码:14203 / +
页数:13
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