Novel photosensitizer for dye-sensitized solar cell based on ionic liquid-doped blend polymer electrolyte

被引：23
|
作者：
Devadiga, Dheeraj [1 ]
Selvakumar, M. [1 ]
Shetty, Prakasha [1 ]
Mahesha, M. G. [2 ]
Devadiga, Deepak [3 ]
Ahipa, T. N. [3 ]
Kumar, S. Senthil [4 ]
机构：
[1] Manipal Acad Higher Educ, Manipal Inst Technol, Dept Chem, Manipal 576104, Karnataka, India
[2] Manipal Acad Higher Educ, Manipal Inst Technol, Dept Phys, Manipal 576104, Karnataka, India
[3] Jain Univ, Ctr Nano & Mat Sci, Jain Global Campus, Bangalore 562112, Karnataka, India
[4] Cent Electrochem Res Inst, CSIR, Elect & Electrocatalysis Div, Karaikkudi 630003, Tamil Nadu, India
来源：
JOURNAL OF SOLID STATE ELECTROCHEMISTRY | 2021年 / 25卷 / 04期
关键词：
Dye-sensitized solar cell; Supercapacitor; Silver doped titanium dioxide; Carbazole based dye; Blend polymer electrolyte; Reduced graphene oxide;
D O I：
10.1007/s10008-021-04920-2
中图分类号：
O646 [电化学、电解、磁化学];
学科分类号：
081704 ;
摘要：
The existing energy situation demands not only the huge energy in a short time but also clean energy. In this regard, an integrated photo-supercapacitor device has been fabricated in which photoelectric conversion and energy storage are achieved simultaneously. A novel carbazole-based dye is synthesized and characterized for photosensitizer. The silver-doped titanium dioxide (Ag-TiO2) is synthesized, and it is used as photoanode material. Different concentrations of tetrabutylammonium iodide (TBAI)-doped polyvinyl alcohol-polyvinylpyrrolidone (PVA-PVP) blend polymer electrolytes are prepared, and their conductivity and dielectric properties were studied. Reduced graphene oxide (r-GO) is synthesized by a one-pot synthesis method and confirmed using Raman spectroscopy for counter electrode material in dye-sensitized solar cell (DSSC) and supercapacitor electrodes. The DSSC having 4% Ag-TiO2-based photoanode showed the highest efficiency of 1.06% (among r-GO counter electrodes) and 2.37% (among platinum counter electrodes). The supercapacitor before integration and after integration exhibits specific capacitance of 1.72 Fg(-1) and 1.327 Fg(-1), respectively.
引用
收藏
页码：1461 / 1478
页数：18
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