Single-crystal neutron diffraction study of short-range magnetic correlations in Tb5Ge4

被引:13
作者
Tian, W. [1 ,2 ]
Kreyssig, A. [1 ,2 ]
Zarestky, J. L. [1 ,2 ]
Tan, L. [1 ,2 ]
Nandi, S. [1 ,2 ]
Goldman, A. I. [1 ,2 ]
Lograsso, T. A. [2 ]
Schlagel, D. L. [2 ]
Gschneidner, K. A. [2 ,3 ]
Pecharsky, V. K. [2 ,3 ]
McQueeney, R. J. [1 ,2 ]
机构
[1] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA
[2] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA
[3] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA
基金
美国能源部;
关键词
REFRIGERATION; BEHAVIOR; ALLOYS;
D O I
10.1103/PhysRevB.80.134422
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We present a single-crystal neutron diffraction study of the magnetic short-range correlations in Tb5Ge4 which orders antiferromagnetically below the Neel temperature T-N approximate to 92 K. Strong diffuse scattering arising from magnetic short-range correlations was observed in wide temperature ranges both below and above T-N. The antiferromagnetic ordering in Tb5Ge4 is described to consist of strongly coupled ferromagnetic block layers in the ac plane that stack along the b axis with weak antiferromagnetic interlayer coupling. Diffuse scattering was observed along both a* and b* directions indicating three-dimensional short-range correlations. Moreover, the q dependence of the diffuse scattering is Squared Lorentzian in form suggesting a strongly clustered magnetic state that may be related to the proposed Griffiths-like phase in Gd5Ge4.
引用
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页数:5
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