Hierarchical nanosheets of ternary CoNiFe layered double hydroxide for supercapacitors and oxygen evolution reaction

被引:54
作者
Rohn, R. C. [1 ]
Jagadale, Ajay D. [1 ]
Shinde, Surendra K. [2 ]
Kim, D-Y [2 ]
Kumbhar, Vijay S. [3 ]
Nakayama, Masaharu [3 ]
机构
[1] SASTRA Deemed Univ, Sch Elect & Elect Engn, Ctr Energy Storage & Convers, Thanjavur 613401, Tamil Nadu, India
[2] Dongguk Univ, Coll Life Sci & Biotechnol, Dept Biol & Environm Sci, 32 Dongguk Ro,Biomed Campus, Goyang Si 10326, Gyeonggi Do, South Korea
[3] Yamaguchi Univ, Grad Sch Sci & Technol Innovat, Dept Appl Chem, 2-16-1 Tokiwadai, Ube, Yamaguchi 7558611, Japan
关键词
Layered double hydroxide; Electrodeposition; Supercapacitor; Electrocatalyst; Oxygen evolution reaction;
D O I
10.1016/j.jallcom.2020.158081
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The preparation of stable and efficient thin films with excellent energy storage and conversion capabilities has attracted great attention in the field of supercapacitors and electrocatalysis. Herein, hierarchical nanosheets-based ternary CoNiFe layered double hydroxide (LDH) thin films are prepared via an inexpensive and facile electrodeposition method. The structural, morphological, and electrochemical properties of films are systematically studied and compared with their binary counterparts. As prepared CoNiFe LDH shows a maximum specific capacity of 360 C g(-1) at the current density of 0.4 A g(-1) with a capacity retention of 51% even at the higher current density of 10 A g(-1). Moreover, it shows excellent cyclic stability of 84% after 2000 cycles. As an electrocatalyst, CoNiFe LDH demonstrates an excellent performance in OER, affording an overpotential of 196 mV at the current density of 10 mA cm(-2) with a Tafel slope value of 49 mV dec(-1). Also, it depicts excellent catalytic stability with stable operation for over 10 h. Thus, ternary CoNiFe LDH thin film can be used as a promising electrode material for both electrochemical energy storage and catalysis. (C) 2020 Elsevier B.V. All rights reserved.
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页数:8
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