Source apportionment of carbonaceous aerosols during haze days in Shanghai based on dual carbon isotopes

被引:7
作者
Wei, Nannan [1 ,2 ]
Xu, Zhiyou [1 ]
Wang, Guanghua [2 ]
Liu, Wei [2 ]
Zhouga, Deqing [3 ]
Xiao, Detao [1 ]
Yao, Jian [2 ]
机构
[1] Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Peoples R China
[2] Chinese Acad Sci, Shanghai Inst Appl Phys, Dept Nucl Reactor Engn, Shanghai 201800, Peoples R China
[3] Tibet Autonomous Reg Meteorol Bur, Meteorol Serv Ctr, Lhasa 850000, Peoples R China
基金
中国国家自然科学基金;
关键词
Fine particulate matter; Organic carbon; Elemental carbon; Delta C-14; delta C-13; SOLUBLE ORGANIC-CARBON; ELEMENTAL CARBON; AMBIENT PM2.5; BLACK CARBON; POLLUTION; WINTER; PARTICULATE; EVENTS; CITIES; VARIABILITY;
D O I
10.1007/s10967-019-06609-3
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
We present dual carbon isotope constrained (delta C-13 and Delta C-14) source apportionment of organic carbon and elemental carbon in fine particulate matter (PM2.5) for five districts of Shanghai during the winter of 2013. The results show that spatial variations of the three source (biomass, liquid fossil fuel, and coal) apportionment of carbonaceous aerosol among different districts were evident. Overall, coal combustion, liquid fossil fuel combustion and biomass burning are the most important carbonaceous aerosols source in Pudong, Xuhui and Chongming, respectively. The results suggest that environmental protection policies should vary according to the functional areas of different sources in the same city.
引用
收藏
页码:383 / 389
页数:7
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