Nonself-Sustained Microwave Discharge in a System for Hydrocarbon Decomposition and Generation of Carbon Nanotubes

被引:9
作者
Korolev, Yury D. [1 ,2 ]
Frants, Oleg B. [1 ]
Landl, Nikolay V. [1 ]
Geyman, Vladimir G. [1 ]
Zerlitsyn, Aleksey G. [3 ]
Shiyan, Vladimir P. [3 ,4 ]
Medvedev, Yury V. [3 ,5 ]
机构
[1] Russian Acad Sci, Inst High Current Elect, Tomsk 634055, Russia
[2] Tomsk State Univ, Tomsk 634050, Russia
[3] Inst Nucl Phys, Tomsk 634050, Russia
[4] Tomsk Polytech Univ, Tomsk 634050, Russia
[5] OAO Tomskgazprom, Tomsk 634009, Russia
基金
俄罗斯基础研究基金会;
关键词
Glow-to-spark transition; microwave discharge; nanotubes; plasma torches;
D O I
10.1109/TPS.2009.2032546
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
This paper deals with the investigation of a method for sustainment of high-power microwave discharge in the installation for natural-gas decomposition. The essence of the method is to provide a generation of auxiliary discharge plasma in the area where the main microwave plasma torch burns. The design of the electrode system of auxiliary discharge resembles that for a coaxial plasmatron that consumes an average current of about 0.1 A. Then, the nonself-sustained microwave discharge with a frequency of 2.45 GHz has been obtained at a power level from 1 to 3 kW. Such a discharge has been used in the installation for natural-gas decomposition and generation of the carbon nanotubes. With a typical gas flow of 1 m(3)/h, the natural-gas conversion achieves 40%-80%. Three types of nanotubes are contained in the final product: multilayer tubes, single-layer tubes, and onion-type tubes.
引用
收藏
页码:2298 / 2302
页数:5
相关论文
共 10 条
[1]   Propane-air mixture combustion assisted by MW discharge in a speedy airflow [J].
Esakov, Igor I. ;
Grachev, Lev P. ;
Khodataev, Kirill V. ;
Vinogradov, Viacheslav A. ;
Van Wie, David M. .
IEEE TRANSACTIONS ON PLASMA SCIENCE, 2006, 34 (06) :2497-2506
[2]   Gliding arc discharges as a source of intermediate plasma for methane partial oxidation [J].
Kalra, CS ;
Gutsol, AF ;
Fridman, AA .
IEEE TRANSACTIONS ON PLASMA SCIENCE, 2005, 33 (01) :32-41
[3]   Hydrogasification of carbon in an atmospheric pressure microwave plasma [J].
Kim, Yongho ;
Abbate, Sara ;
Ziock, Hans ;
Anderson, Graydon K. ;
Rosocha, Louis A. .
IEEE TRANSACTIONS ON PLASMA SCIENCE, 2007, 35 (06) :1677-1681
[4]   Glow-to-spark transitions in a plasma system for ignition and combustion control [J].
Korolev, Yury D. ;
Frants, Oleg B. ;
Landl, Nikolay V. ;
Geyman, Vladimir G. ;
Matveev, Igor B. .
IEEE TRANSACTIONS ON PLASMA SCIENCE, 2007, 35 (06) :1651-1657
[5]   Nonsteady-State Gas-Discharge Processes in Plasmatron for Combustion Sustaining and Hydrocarbon Decomposition [J].
Korolev, Yury D. ;
Frants, Oleg B. ;
Landl, Nikolay V. ;
Geyman, Vladimir G. ;
Matveev, Igor B. .
IEEE TRANSACTIONS ON PLASMA SCIENCE, 2009, 37 (04) :586-592
[6]  
KOSSYI IA, 2006, 44 AIAA AER SCI M EX
[7]  
MEDVEDEV YV, 2008, Patent No. 2317943
[8]   Determination of the electrical parameters of a bi-dimensional dc Glidarc [J].
Pellerin, S ;
Cormier, JM ;
Richard, F ;
Musiol, K ;
Chapelle, J .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 1999, 32 (08) :891-897
[9]  
ROSOCHA LA, 2006, PLASMA PHYS APPL, pCH3
[10]  
WARANTZ J, 2001, COMBUSTION PHYS CHEM