Ultrafast extreme rejuvenation of metallic glasses by shock compression

被引:100
作者
Ding, G. [1 ,2 ]
Li, C. [1 ,3 ]
Zaccone, A. [4 ,5 ,6 ]
Wang, W. H. [7 ]
Lei, H. C. [8 ]
Jiang, F. [2 ]
Ling, Z. [1 ]
Jiang, M. Q. [1 ,3 ]
机构
[1] Chinese Acad Sci, Inst Mech, State Key Lab Nonlinear Mech, Beijing 100190, Peoples R China
[2] Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Xian 710049, Shaanxi, Peoples R China
[3] Univ Chinese Acad Sci, Sch Engn Sci, Beijing 100049, Peoples R China
[4] Univ Milan, Dept Phys, Via Celoria 16, I-20133 Milan, Italy
[5] Univ Cambridge, Dept Chem Engn & Biotechnol, Cambridge CB2 3RA, England
[6] Univ Cambridge, Cavendish Lab, Cambridge CB3 9HE, England
[7] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China
[8] Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China
基金
中国国家自然科学基金;
关键词
AMORPHOUS ALLOY; STRUCTURAL RELAXATION; SHEAR BANDS; FREE-VOLUME; LIQUIDS; DEFORMATION; PLASTICITY; DYNAMICS; STRENGTH; ORIGIN;
D O I
10.1126/sciadv.aaw6249
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Structural rejuvenation of glasses not only provides fundamental insights into their complicated dynamics but also extends their practical applications. However, it is formidably challenging to rejuvenate a glass on very short time scales. Here, we present the first experimental evidence that a specially designed shock compression technique can rapidly rejuvenate metallic glasses to extremely high-enthalpy states within a very short time scale of about 365 +/- 8 ns. By controlling the shock stress amplitude, the shock-induced rejuvenation is successfully frozen at different degrees. The underlying structural disordering is quantitatively characterized by the anomalous boson heat capacity peak of glasses. A Deborah number, defined as a competition of time scales between the net structural disordering and the applied loading, is introduced to explain the observed ultrafast rejuvenation phenomena of metallic glasses.
引用
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页数:7
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