Synthesis of Au@UiO-66(NH2) structures by small molecule-assisted nucleation for plasmon-enhanced photocatalytic activity

被引:105
作者
Gu, Zhizhi [1 ]
Chen, Liyong [1 ]
Duan, Binhua [1 ]
Luo, Qiong [1 ]
Liu, Jing [1 ]
Duan, Chunying [1 ]
机构
[1] Dalian Univ Technol, State Key Lab Fine Chem, Dalian 116024, Peoples R China
基金
中国国家自然科学基金; 高等学校博士学科点专项科研基金;
关键词
METAL-ORGANIC FRAMEWORKS; ELECTRON-TRANSFER; NANOPARTICLES; CATALYSTS; MOFS; REDUCTION; AU;
D O I
10.1039/c5cc07042b
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We have provided a small molecule-assisted heterogeneous nucleation of MOF route to successfully synthesize Au@UiO-66(NH2) heterostructures. UiO-66(NH2) with a localized electronic state that was characterized by C-AFM exhibited higher photocatalytic activity in the heterostructures via a plasmonic sensitization process.
引用
收藏
页码:116 / 119
页数:4
相关论文
共 23 条
[1]   Synthesis of Au@ZIF-8 single- or multi-core-shell structures for photocatalysis [J].
Chen, Liyong ;
Peng, Yan ;
Wang, Hong ;
Gua, Zhizhi ;
Duan, Chunying .
CHEMICAL COMMUNICATIONS, 2014, 50 (63) :8651-8654
[2]   Catalysis of Transesterification by a Nonfunctionalized Metal-Organic Framework: Acido-Basicity at the External Surface of ZIF-8 Probed by FTIR and ab Initio Calculations [J].
Chizallet, Celine ;
Lazare, Sandrine ;
Bazer-Bachi, Delphine ;
Bonnier, Fabien ;
Lecocq, Vincent ;
Soyer, Emmanuel ;
Quoineaud, Anne-Agathe ;
Bats, Nicolas .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2010, 132 (35) :12365-12377
[3]   Higher-order organization by mesoscale self-assembly and transformation of hybrid nanostructures [J].
Cölfen, H ;
Mann, S .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2003, 42 (21) :2350-2365
[4]   Catalysis by metal nanoparticles embedded on metal-organic frameworks [J].
Dhakshinamoorthy, Amarajothi ;
Garcia, Hermenegildo .
CHEMICAL SOCIETY REVIEWS, 2012, 41 (15) :5262-5284
[5]   Using Functional Nano- and Microparticles for the Preparation of Metal-Organic Framework Composites with Novel Properties [J].
Doherty, Cara M. ;
Buso, Dario ;
Hill, Anita J. ;
Furukawa, Shuhei ;
Kitagawa, Susumu ;
Falcaro, Paolo .
ACCOUNTS OF CHEMICAL RESEARCH, 2014, 47 (02) :396-405
[6]   An Amine-Functionalized Titanium Metal-Organic Framework Photocatalyst with Visible-Light-Induced Activity for CO2 Reduction [J].
Fu, Yanghe ;
Sun, Dengrong ;
Chen, Yongjuan ;
Huang, Renkun ;
Ding, Zhengxin ;
Fu, Xianzhi ;
Li, Zhaohui .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2012, 51 (14) :3364-3367
[7]   Au@UiO-66: a base free oxidation catalyst [J].
Leus, K. ;
Concepcion, P. ;
Vandichel, M. ;
Meledina, M. ;
Grirrane, A. ;
Esquivel, D. ;
Turner, S. ;
Poelman, D. ;
Waroquier, M. ;
Van Speybroeck, V. ;
Van Tendeloo, G. ;
Garcia, H. ;
Van Der Voort, P. .
RSC ADVANCES, 2015, 5 (29) :22334-22342
[8]   Core-Shell Upconversion Nanoparticle@Metal-Organic Framework Nanoprobes for Luminescent/Magnetic Dual-Mode Targeted Imaging [J].
Li, Yantao ;
Tang, Jinglong ;
He, Liangcan ;
Liu, Yong ;
Liu, Yaling ;
Chen, Chunying ;
Tang, Zhiyong .
ADVANCED MATERIALS, 2015, 27 (27) :4075-4080
[9]   Feasible synthesis of etched gold nanoplates with catalytic activity and SERS properties [J].
Liu, Hongyu ;
Yang, Qing .
CRYSTENGCOMM, 2011, 13 (17) :5488-5494
[10]   Amine-functionalized zirconium metal-organic framework as efficient visible-light photocatalyst for aerobic organic transformations [J].
Long, Jinlin ;
Wang, Sibo ;
Ding, Zhengxin ;
Wang, Shuchao ;
Zhou, Yangen ;
Huang, Ling ;
Wang, Xuxu .
CHEMICAL COMMUNICATIONS, 2012, 48 (95) :11656-11658