Dynamics of one-dimensional and two-dimensional helium adsorbed on carbon nanotubes

被引:10
作者
Diallo, S. O. [1 ,2 ]
Fak, B. [3 ]
Adams, M. A. [4 ]
Vilches, O. E. [5 ]
Johnson, M. R. [6 ]
Schober, H. [6 ]
Glyde, H. R. [2 ]
机构
[1] Iowa State Univ, Ames Lab, Ames, IA 50011 USA
[2] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA
[3] Commissariat Energie Atom, INAC, SPSMS, F-38054 Grenoble, France
[4] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England
[5] Univ Washington, Dept Phys, Seattle, WA 98195 USA
[6] Inst Laue Langevin, F-38042 Grenoble, France
基金
美国国家科学基金会;
关键词
ANDERSON LOCALIZATION; HE-4; FILMS; NEUTRON-SCATTERING; MONTE-CARLO; BUNDLES; FLUIDS; PHASE; NANOPORES; DISORDER; LATTICES;
D O I
10.1209/0295-5075/88/56005
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We present inelastic neutron scattering measurements of the dynamics of helium adsorbed on carbon nanotube bundles. The goal is to determine the vibrational properties of the 1D and 2D quantum solids that are stabilized on the nanotube bundle surfaces at different fillings of (4)He. The mean square vibrational amplitude in the 1D solid is large with a Lindemann ratio of gamma(1D) =(< u2 >)(1/2)/a(1) = 0.25 comparable to bulk solid (4)He. The gamma(2D) is significantly smaller. The frequency density of states of the 2D solid, g(omega), has a gap at omega similar or equal to 0.75 meV consistent with a commensurate lattice. The 1D solid has no gap or a gap smeared by disorder. The 1D and 2D g(omega) are well described by dispersion curves having no gap and a gap, respectively, with some vibration along additional dimensions indicated. Copyright (C) EPLA, 2009
引用
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页数:6
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