Modeling study of the 2010 regional haze event in the North China Plain

被引:190
作者
Gao, M. [1 ,2 ]
Carmichael, G. R. [1 ,2 ]
Wang, Y. [3 ]
Saide, P. E. [2 ,4 ]
Yu, M. [1 ,2 ,5 ]
Xin, J. [3 ]
Liu, Z. [3 ]
Wang, Z. [3 ]
机构
[1] Univ Iowa, Dept Chem & Biochem Engn, Iowa City, IA 52242 USA
[2] Univ Iowa, Ctr Global & Reg Environm Res, Iowa City, IA USA
[3] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & At, Beijing, Peoples R China
[4] Natl Ctr Atmospher Res, Atmospher Chem Observat & Modeling ACOM Lab, POB 3000, Boulder, CO 80307 USA
[5] Argonne Natl Lab, Math & Comp Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA
基金
中国国家自然科学基金;
关键词
SECONDARY ORGANIC AEROSOL; URBAN AIR-QUALITY; FORMATION MECHANISM; SOUTHERN HEBEI; EASTERN CHINA; WINTER HAZE; POLLUTION; IMPACT; TRANSPORT; EPISODE;
D O I
10.5194/acp-16-1673-2016
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The online coupled Weather Research and Forecasting-Chemistry (WRF-Chem) model was applied to simulate a haze event that happened in January 2010 in the North China Plain (NCP), and was validated against various types of measurements. The evaluations indicate that WRF-Chem provides reliable simulations for the 2010 haze event in the NCP. This haze event was mainly caused by high emissions of air pollutants in the NCP and stable weather conditions in winter. Secondary inorganic aerosols also played an important role and cloud chemistry had important contributions. Air pollutants outside Beijing contributed about 64.5% to the PM2.5 levels in Beijing during this haze event, and most of them are from south Hebei, Tianjin city, Shandong and Henan provinces. In addition, aerosol feedback has important impacts on surface temperature, relative humidity (RH) and wind speeds, and these meteorological variables affect aerosol distribution and formation in turn. In Shijiazhuang, Planetary Boundary Layer (PBL) decreased about 278.2 m and PM2.5 increased more than 20 mu g m(-3) due to aerosol feedback. It was also shown that black carbon (BC) absorption has significant impacts on meteorology and air quality changes, indicating more attention should be paid to BC from both air pollution control and climate change perspectives.
引用
收藏
页码:1673 / 1691
页数:19
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