Enabling large-scale hydrogen storage in porous media - the scientific challenges

被引:580
作者
Heinemann, Niklas [1 ]
Alcalde, Juan [2 ]
Miocic, Johannes M. [3 ,4 ]
Hangx, Suzanne J. T. [5 ]
Kallmeyer, Jens [6 ]
Ostertag-Henning, Christian [7 ]
Hassanpouryouzband, Aliakbar [1 ]
Thaysen, Eike M. [1 ]
Strobel, Gion J. [8 ]
Schmidt-Hattenberger, Cornelia [6 ]
Edlmann, Katriona [1 ]
Wilkinson, Mark [1 ]
Bentham, Michelle [9 ]
Haszeldine, R. Stuart [1 ]
Carbonell, Ramon [2 ]
Rudloff, Alexander [6 ]
机构
[1] Univ Edinburgh, Sch Geosci, Edinburgh, Midlothian, Scotland
[2] CSIC, Geosci Barcelona, Barcelona, Spain
[3] Univ Freiburg, Inst Earth & Environm Sci, Freiburg, Germany
[4] Univ Groningen, Energy & Sustainabil Res Inst Groningen ESRIG, Groningen, Netherlands
[5] Univ Utrecht, Dept Earth Sci, Utrecht, Netherlands
[6] GFZ German Res Ctr Geosci, Potsdam, Germany
[7] Fed Inst Geosci & Nat Resources, Hannover, Germany
[8] Tech Univ Clausthal, Inst Subsurface Energy Syst, Clausthal Zellerfeld, Germany
[9] British Geol Survey, Nottingham, England
基金
英国工程与自然科学研究理事会;
关键词
UNDERGROUND GAS-STORAGE; NATURAL-GAS; METHANOGENIC BACTERIA; CO2; STORAGE; SP-NOV; NUMERICAL-SIMULATION; ENERGY-STORAGE; CARBON-DIOXIDE; DEPLETED OIL; REDUCTION;
D O I
10.1039/d0ee03536j
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Expectations for energy storage are high but large-scale underground hydrogen storage in porous media (UHSP) remains largely untested. This article identifies and discusses the scientific challenges of hydrogen storage in porous media for safe and efficient large-scale energy storage to enable a global hydrogen economy. To facilitate hydrogen supply on the scales required for a zero-carbon future, it must be stored in porous geological formations, such as saline aquifers and depleted hydrocarbon reservoirs. Large-scale UHSP offers the much-needed capacity to balance inter-seasonal discrepancies between demand and supply, decouple energy generation from demand and decarbonise heating and transport, supporting decarbonisation of the entire energy system. Despite the vast opportunity provided by UHSP, the maturity is considered low and as such UHSP is associated with several uncertainties and challenges. Here, the safety and economic impacts triggered by poorly understood key processes are identified, such as the formation of corrosive hydrogen sulfide gas, hydrogen loss due to the activity of microbes or permeability changes due to geochemical interactions impacting on the predictability of hydrogen flow through porous media. The wide range of scientific challenges facing UHSP are outlined to improve procedures and workflows for the hydrogen storage cycle, from site selection to storage site operation. Multidisciplinary research, including reservoir engineering, chemistry, geology and microbiology, more complex than required for CH4 or CO2 storage is required in order to implement the safe, efficient and much needed large-scale commercial deployment of UHSP.
引用
收藏
页码:853 / 864
页数:12
相关论文
共 155 条
[1]   Estimating geological CO2 storage security to deliver on climate mitigation [J].
Alcalde, Juan ;
Flude, Stephanie ;
Wilkinson, Mark ;
Johnson, Gareth ;
Edlmann, Katriona ;
Bond, Clare E. ;
Scott, Vivian ;
Gilfillan, Stuart M. V. ;
Ogaya, Xenia ;
Haszeldine, R. Stuart .
NATURE COMMUNICATIONS, 2018, 9
[2]  
[Anonymous], 2020, Fuel Cells and Hydrogen 2 Joint Undertaking
[3]  
[Anonymous], Intergovernmental Panel on Climate Change
[4]  
ARENA (Australian Renewable Energy Agency), REN HYDR DEPL FUND R
[5]   STRESS-CORROSION CRACKING OF QUARTZ - A NOTE ON THE INFLUENCE OF CHEMICAL ENVIRONMENT [J].
ATKINSON, BK ;
MEREDITH, PG .
TECTONOPHYSICS, 1981, 77 (1-2) :T1-T11
[6]   Hydrogen uptake and diffusion in Callovo-Oxfordian clay rock for nuclear waste disposal technology [J].
Bardelli, Fabrizio ;
Mondelli, Claudia ;
Didier, Mathilde ;
Vitillo, Jenny G. ;
Cavicchia, Demetrio R. ;
Robinet, Jean-Charles ;
Leone, Laura ;
Charlet, Laurent .
APPLIED GEOCHEMISTRY, 2014, 49 :168-177
[7]  
Bauer S, 2018, UNDERGROUND SUN CONV
[8]   Geochemical Effects of Millimolar Hydrogen Concentrations in Groundwater: An Experimental Study in the Context of Subsurface Hydrogen Storage [J].
Berta, Marton ;
Dethlefsen, Frank ;
Ebert, Markus ;
Schaefer, Dirk ;
Dahmke, Andreas .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2018, 52 (08) :4937-4949
[9]  
Blunt MJ, 2017, MULTIPHASE FLOW PERM, DOI DOI 10.1017/9781316145098
[10]   Radioisotopic, culture-based, and oligonucleotide microchip analyses of thermophilic microbial communities in a continental high-temperature petroleum reservoir [J].
Bonch-Osmolovskaya, EA ;
Miroshnichenko, ML ;
Lebedinsky, AV ;
Chernyh, NA ;
Nazina, TN ;
Ivoilov, VS ;
Belyaev, SS ;
Boulygina, ES ;
Lysov, YP ;
Perov, AN ;
Mirzabekov, AD ;
Hippe, H ;
Stackebrandt, E ;
L'Haridon, S ;
Jeanthon, C .
APPLIED AND ENVIRONMENTAL MICROBIOLOGY, 2003, 69 (10) :6143-6151