Passivation and process engineering approaches of halide perovskite films for high efficiency and stability perovskite solar cells

被引:260
作者
Mohd Yusoff, Abd. Rashid bin [1 ]
Vasilopoulou, Maria [2 ]
Georgiadou, Dimitra G. [3 ,4 ]
Palilis, Leonidas C. [5 ]
Abate, Antonio [6 ,7 ,8 ]
Nazeeruddin, Mohammad Khaja [9 ]
机构
[1] Pohang Univ Sci & Technol POSTECH, Dept Chem Engn, Pohang 37673, Gyeongbuk, South Korea
[2] Natl Ctr Sci Res Demokritos, Inst Nanosci & Nanotechnol, Aghia Paraskevi 15341, Attica, Greece
[3] Univ Southampton, Zepler Inst Photon & Nanoelect, Ctr Elect Frontiers, Southampton SO17 1BJ, Hants, England
[4] Imperial Coll London, Dept Phys, London SW7 2AZ, England
[5] Univ Patras, Dept Phys, Patras 26504, Greece
[6] Helmholtz Zentrum Berlin Mat & Energie, Kekulestr 5, D-12489 Berlin, Germany
[7] Univ Naples Federico II, Dept Chem Mat & Prod Engn, Piazzale Tecchio 80, I-80125 Fuorigrotta, Italy
[8] Fuzhou Univ, Inst Adv Energy Mat, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Fujian, Peoples R China
[9] Ecole Polytech Fed Lausanne EPFL, Inst Chem Sci & Engn, Grp Mol Engn Funct Mat, Rue Ind 17, CH-1951 Sion, Switzerland
关键词
LOW-TEMPERATURE CRYSTALLIZATION; POWER CONVERSION EFFICIENCY; CHARGE-CARRIER DYNAMICS; LONG-TERM STABILITY; DEFECT-PASSIVATION; 2-DIMENSIONAL PEROVSKITE; SURFACE PASSIVATION; INDUCED DEGRADATION; GRAIN-BOUNDARY; THIN-FILMS;
D O I
10.1039/d1ee00062d
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The surface, interfaces and grain boundaries of a halide perovskite film carry critical tasks in achieving as well as maintaining high solar cell performance due to the inherently defective nature across their regime. Passivating materials and felicitous process engineering approaches have significant ramifications in the resultant perovskite film, and the solar cell's overall macroscale properties as they dictate structural and optoelectronic properties. Herein, we exploit a vast number of defect engineering approaches aiming to increase the performance and the stability of perovskite solar cells, especially against humidity, continuous illumination, and heat. This review begins with the perovskite materials' fundamental structural properties followed by the advances made to induce higher stabilization in perovskite solar cells by fine-tuning materials chemistry design parameters. We continue by summarizing defect passivation strategies based on molecular entities' application, including suitable functional groups that enable sufficient surface, bulk and grain boundary passivation, morphology, and crystallinity control. We also present methods to control the density of defects through the variation of processing conditions, solvent annealing and solvent engineering approaches, gas-assisted deposition methods, and use of self-assembled monolayers, as well as colloidal engineering and coordination surface chemistry. Finally, we give our perspective on how a combined understanding of materials chemistry aspects and passivation mechanisms will further develop high-efficiency and stability perovskite solar cells.
引用
收藏
页码:2906 / 2953
页数:48
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