One-step solution synthesis of a two-dimensional semiconducting covalent organometallic nanosheet via the condensation of boronic acid

被引:2
|
作者
Wang, Qijun [1 ]
Yan, Jiahao [2 ]
Xiao, Mingchao [1 ,3 ]
Manoj, Devaraj [1 ]
Zhong, Cheng [5 ]
Lv, Qiying [1 ]
Yang, Lite [1 ]
Wu, Liangmei [2 ]
Wang, Zhuoping [1 ]
Bao, Lihong [2 ]
Gao, Hongjun [2 ]
Xiao, Fei [1 ]
Jiang, Lang [3 ]
Wang, Shuai [1 ,4 ]
机构
[1] Huazhong Univ Sci & Technol, Sch Chem & Chem Engn, Wuhan 430074, Hubei, Peoples R China
[2] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China
[3] Chinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China
[4] Fudan Univ, Dept Mat Sci, Shanghai 200433, Peoples R China
[5] Wuhan Univ, Coll Chem & Mol Sci, Wuhan 430072, Hubei, Peoples R China
基金
中国国家自然科学基金;
关键词
ORGANIC FRAMEWORKS; CRYSTALLINE; POLYMER;
D O I
10.1039/c9ra05806k
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In this work, a 2D covalent organometallic nanosheet (COMS) was designed and successfully synthesized through the one-step conjunction of a terpyridine-metal-terpyridine (TMT) sandwich coordinate motif with borate ester covalent heterocyclic (B3O3) linkage via the condensation of boronic acid. The obtained 2D COMS with a cobalt coordination center (2D COMS-Co) showed promising p-type semiconducting properties.
引用
收藏
页码:29327 / 29330
页数:4
相关论文
共 50 条
  • [41] A new approach in the one-step synthesis of α-MnO2via a modified solution combustion procedure
    Moqaddam, Mahsa Mohammadi
    Mirjalili, Mostafa
    Khaki, Jalil Vahdati
    Beidokhti, Sahar Mollazadeh
    NANOSCALE ADVANCES, 2022, 4 (18): : 3909 - 3918
  • [42] Facile synthesis of aryl-triazine linked two-dimensional covalent organic frameworks via ?two-in-one? strategy for phenolic compounds adsorption
    Zhou, Chengda
    Zhou, Huyan
    Tang, Shiyun
    Zhang, Fengmei
    Lei, Sheng
    Li, Zhenjie
    Chen, Mao
    Liu, Jingjing
    MATERIALS LETTERS, 2023, 332
  • [43] A mild and one-step synthesis of 2,8-dioxabicyclo [3.3.1] nonane derivatives via classical Knoevenagel condensation
    Yang, De-Suo
    Ke, Sen
    Du, Xin
    Gao, Peng
    Zhu, Hai-Tao
    Fan, Ming-Jin
    TETRAHEDRON, 2017, 73 (37) : 5522 - 5527
  • [44] Catalytic Atroposelective Synthesis of Axially Chiral Heterobiaryl Oxime Ethers via the One-Step Dynamic Kinetic Condensation Reaction
    Xu, Qianqian
    Jia, Jifan
    Fan, Haitong
    Ma, Zhifeng
    Wu, Yuqing
    Zhang, Yifeng
    Su, Ping
    Gao, Wei
    Wang, Yuji
    Li, Dan
    ORGANIC LETTERS, 2024, 26 (12) : 2403 - 2408
  • [45] One-Step Butadiene Synthesis via Gas-Phase Prins Condensation of Propylene with Formaldehyde over Heteropolyacid Catalysts
    Kots, Pavel A.
    Artsiusheuski, Mikalai A.
    Grigoriev, Yuriy, V
    Ivanova, Irina I.
    ACS CATALYSIS, 2020, 10 (24) : 15149 - 15161
  • [46] ONE-STEP SYNTHESIS OF ISOPRENE BY VAPOR-PHASE CONDENSATION OF FORMALDEHYDE WITH ISOBUTYLENE OVER BORIC-ACID CATALYSTS
    YASHIMA, T
    OHARA, T
    YOKOI, N
    HARA, N
    NIPPON KAGAKU KAISHI, 1974, (02) : 325 - 330
  • [47] Synthesis of a Scalable Two-Dimensional Covalent Organic Framework by the Photon-Assisted (mine Condensation Reaction on the Water Surface
    Kim, Soyoung
    Lim, Hyunseob
    Lee, Jinho
    Choi, Hee Cheul
    LANGMUIR, 2018, 34 (30) : 8731 - 8738
  • [48] Synthesis and photocatalytic activity of ultrathin two-dimensional porphyrin nanodisks via covalent organic framework exfoliation
    Zeyu Fan
    Kota Nomura
    Mingshan Zhu
    Xinxi Li
    Jiawei Xue
    Tetsuro Majima
    Yasuko Osakada
    Communications Chemistry, 2
  • [49] Synthesis and photocatalytic activity of ultrathin two-dimensional porphyrin nanodisks via covalent organic framework exfoliation
    Fan, Zeyu
    Nomura, Kota
    Zhu, Mingshan
    Li, Xinxi
    Xue, Jiawei
    Majima, Tetsuro
    Osakada, Yasuko
    COMMUNICATIONS CHEMISTRY, 2019, 2
  • [50] Synthesis and characterization of Fe-Co binary ferrospinel nanospheres via one-step nonaqueous solution pathway
    Jiang, J.
    Ai, L. H.
    MATERIALS LETTERS, 2010, 64 (08) : 945 - 947