Weakening of the weekend ozone effect over California's South Coast Air Basin

被引:35
作者
Baidar, S. [1 ,2 ]
Hardesty, R. M. [2 ,3 ]
Kim, S-W. [2 ,3 ]
Langford, A. O. [3 ]
Oetjen, H. [1 ]
Senff, C. J. [2 ,3 ]
Trainer, M. [3 ]
Volkamer, R. [1 ,2 ]
机构
[1] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA
[2] Univ Colorado, CIRES, Boulder, CO 80309 USA
[3] NOAA Earth Syst Res Lab, Div Chem Sci, Boulder, CO USA
关键词
MOTOR-VEHICLE EMISSIONS; SAN-JOAQUIN VALLEY; LOS-ANGELES BASIN; AEROSOL EXTINCTION; NITROGEN-OXIDES; WEEKDAY; NO2; REDUCTIONS; REACTIVITY; POLLUTION;
D O I
10.1002/2015GL066419
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
We have observed lower nitrogen dioxide (NO2) and ozone (O-3) during a hot weekend (summer 2010) from aircraft over the entire South Coast Air Basin (SoCAB). Surface concentrations of NO2, O-3, and temperature from 1996 to 2014 corroborate that this lower O-3 on weekends is increasingly likely in recent years. While higher surface O-3 on the weekends (weekend ozone effect, WO3E) remains widespread, the spatial extent and the trend in the probability of WO3E occurrences (P-WO3E) have decreased significantly compared to a decade ago. This decrease is mostly the result of lower O-3 on hot weekends in recent years. P-WO3E is lowest in the eastern SoCAB. The major decrease happened during the 2008 economic recession, after which P-WO3E has stabilized at a 15-25% lower level throughout most of the basin. Future NOx reductions are likely to be increasingly effective at reducing O-3 pollution initially under hot conditions in the coming decade.
引用
收藏
页码:9457 / 9464
页数:8
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