Design of hollow carbon-based materials derived from metal-organic frameworks for electrocatalysis and electrochemical energy storage

被引:143
作者
Hu, Wenhui [1 ]
Zheng, Mingbo [1 ]
Xu, Bingyan [1 ]
Wei, Ying [1 ]
Zhu, Wei [1 ]
Li, Qing [2 ]
Pang, Huan [1 ]
机构
[1] Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Jiangsu, Peoples R China
[2] Yangzhou Univ, Guangling Coll, Yangzhou 225128, Jiangsu, Peoples R China
基金
中国国家自然科学基金;
关键词
OXYGEN EVOLUTION REACTION; DOPED POROUS CARBON; ELECTROLYTE INTERPHASE LAYER; SODIUM-ION BATTERIES; HIGH-PERFORMANCE; ANODE MATERIALS; BIFUNCTIONAL ELECTROCATALYST; EFFICIENT ELECTROCATALYST; ACTIVATED CARBON; HIGHLY EFFICIENT;
D O I
10.1039/d0ta10666f
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Hollow nanostructured materials are suitable for electrochemical reactions because of their unique internal cavity and short transport path. Carbon-based nanomaterials, including simplex carbon materials, heteroatom-doped carbon materials, carbon-transition metal nanoparticle composites, and carbon-transition metal compound composites, are promising electrode materials because of their high conductivity and stable structure. Hollow carbon-based nanomaterials, which possess the features of the aforementioned materials, have become a research hotspot in electrochemical energy storage and electrocatalysis. The excellent characteristics of metal-organic frameworks (MOFs) make them an ideal material for constructing hollow carbon-based nanomaterials. In this article, the process of preparing MOF-derived hollow carbon-based materials and their applications in electrochemical energy storage and electrocatalysis are reviewed. First, the various methods for preparing MOF-derived hollow carbon-based materials are introduced, and the characteristics of each method are analyzed. Second, the applications of MOF-derived hollow carbon-based materials in the oxygen evolution reaction, oxygen reduction reaction, hydrogen evolution reaction, lithium-ion batteries, sodium-ion batteries, lithium-sulfur batteries, and supercapacitors are analyzed and summarized. Finally, research directions for further development of MOF-derived hollow carbon-based materials are proposed.
引用
收藏
页码:3880 / 3917
页数:38
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