Universal mobility characteristics of graphene originating from charge scattering by ionised impurities

被引:100
作者
Gosling, Jonathan H. [1 ,2 ]
Makarovsky, Oleg [1 ]
Wang, Feiran [2 ]
Cottam, Nathan D. [1 ]
Greenaway, Mark T. [3 ]
Patane, Amalia [1 ]
Wildman, Ricky D. [2 ]
Tuck, Christopher J. [2 ]
Turyanska, Lyudmila [2 ]
Fromhold, T. Mark [1 ]
机构
[1] Univ Nottingham, Sch Phys & Astron, Nottingham NG7 2RD, England
[2] Univ Nottingham, Fac Engn, Ctr Addit Mfg, Nottingham NG7 2RD, England
[3] Loughborough Univ, Dept Phys, Loughborough LE11 3TU, Leics, England
基金
欧盟地平线“2020”; 英国工程与自然科学研究理事会;
关键词
DER-WAALS HETEROSTRUCTURES; 2-DIMENSIONAL MATERIALS; TRANSPORT; LAYER;
D O I
10.1038/s42005-021-00518-2
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Pristine graphene and graphene-based heterostructures can exhibit exceptionally high electron mobility if their surface contains few electron-scattering impurities. Mobility directly influences electrical conductivity and its dependence on the carrier density. But linking these key transport parameters remains a challenging task for both theorists and experimentalists. Here, we report numerical and analytical models of carrier transport in graphene, which reveal a universal connection between graphene's carrier mobility and the variation of its electrical conductivity with carrier density. Our model of graphene conductivity is based on a convolution of carrier density and its uncertainty, which is verified by numerical solution of the Boltzmann transport equation including the effects of charged impurity scattering and optical phonons on the carrier mobility. This model reproduces, explains, and unifies experimental mobility and conductivity data from a wide range of samples and provides a way to predict a priori all key transport parameters of graphene devices. Our results open a route for controlling the transport properties of graphene by doping and for engineering the properties of 2D materials and heterostructures.
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页数:8
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