Coarsening of bicontinuous structures via nonconserved and conserved dynamics

被引:46
作者
Kwon, Yongwoo
Thornton, Katsuyo
Voorhees, Peter W.
机构
[1] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA
[2] Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI 48109 USA
来源
PHYSICAL REVIEW E | 2007年 / 75卷 / 02期
关键词
D O I
10.1103/PhysRevE.75.021120
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
Coarsening subsequent to phase separations occurs in many two-phase mixtures. While unique scaled particle size distributions have been determined for highly asymmetric mixtures in which spherical particles form in a matrix, it is not known if a unique scaled structure exists for symmetric mixtures, which yield bicontinuous structures having intricately interpenetrating phase domains. Using large-scale simulations, we have established that unique scaled microstructures exist in symmetric mixtures evolving via nonconserved and conserved dynamics. We characterize their morphologies by the interfacial shape distribution, a counterpart to the particle size distribution, and their topologies by the genus. We find that the two dynamics result in unique, but different, scaled interfacial shape distributions, with conserved dynamics yielding a narrower distribution around zero mean curvature. In contrast, the two scaled structures are topologically similar, having nearly equal values of the scaled genus.
引用
收藏
页数:5
相关论文
共 32 条
[1]   Scaling properties of the morphological measures at the early and intermediate stages of the spinodal decomposition in homopolymer blends [J].
Aksimentiev, A ;
Moorthi, K ;
Holyst, R .
JOURNAL OF CHEMICAL PHYSICS, 2000, 112 (13) :6049-6062
[2]   Three-dimensional characterization of dendritic microstructures [J].
Alkemper, J ;
Voorhees, PW .
ACTA MATERIALIA, 2001, 49 (05) :897-902
[3]   MICROSCOPIC THEORY FOR ANTIPHASE BOUNDARY MOTION AND ITS APPLICATION TO ANTIPHASE DOMAIN COARSENING [J].
ALLEN, SM ;
CAHN, JW .
ACTA METALLURGICA, 1979, 27 (06) :1085-1095
[4]   Numerical confirmation of late-time t1/2 growth in three-dimensional phase ordering [J].
Brown, Gregory ;
Rikvold, Per Arne .
Physical Review E - Statistical, Nonlinear, and Soft Matter Physics, 2002, 65 (03) :1-036137
[5]   ON SPINODAL DECOMPOSITION [J].
CAHN, JW .
ACTA METALLURGICA, 1961, 9 (09) :795-801
[6]   FREE ENERGY OF A NONUNIFORM SYSTEM .1. INTERFACIAL FREE ENERGY [J].
CAHN, JW ;
HILLIARD, JE .
JOURNAL OF CHEMICAL PHYSICS, 1958, 28 (02) :258-267
[7]   EXPERIMENTAL COARSENING OF ANTIPHASE DOMAINS IN A SILICATE MINERAL [J].
CARPENTER, MA .
SCIENCE, 1979, 206 (4419) :681-683
[8]   ANGULAR-DISTRIBUTION OF LIGHT SCATTERED FROM CRITICALLY QUENCHED LIQUID-MIXTURES [J].
CHOU, YC ;
GOLDBURG, WI .
PHYSICAL REVIEW A, 1981, 23 (02) :858-864
[9]   BICONTINUOUS STRUCTURE ZONES IN MICRO-EMULSIONS [J].
CLAUSSE, M ;
PEYRELASSE, J ;
HEIL, J ;
BONED, C ;
LAGOURETTE, B .
NATURE, 1981, 293 (5834) :636-638
[10]  
Davidovitch B, 2004, PHYS REV E, V70, DOI 10.1103/PhysRevE.70.031609