Particulate matter pollution over China and the effects of control policies

被引:278
作者
Wang, Jiandong [1 ,2 ]
Zhao, Bin [3 ]
Wang, Shuxiao [1 ,2 ]
Yang, Fumo [4 ,5 ]
Xing, Jia [1 ,2 ]
Morawska, Lidia [6 ]
Ding, Aijun [7 ]
Kulmala, Markku [8 ]
Kerminen, Veli-Matti [8 ]
Kujansuu, Joni [8 ]
Wang, Zifa [9 ]
Ding, Dian [1 ,2 ]
Zhang, Xiaoye [10 ]
Wang, Huanbo [4 ]
Tian, Mi [4 ]
Petaja, Tuukka [8 ]
Jiang, Jingkun [1 ,2 ]
Hao, Jiming [1 ,2 ]
机构
[1] Tsinghua Univ, State Key Joint Lab Environm Simulat & Pollut Con, Sch Environm, Beijing 100084, Peoples R China
[2] State Environm Protect Key Lab Sources & Control, Air Pollut Complex, Beijing 100084, Peoples R China
[3] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Joint Inst Reg Earth Syst Sci & Engn, Los Angeles, CA 90095 USA
[4] Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China
[5] Chinese Acad Sci, Inst Urban Environm, Ctr Excellence Reg Atmospher Environm, Xiamen 361021, Peoples R China
[6] Queensland Univ Technol, Int Lab Air Qual & Hlth, GPO Box 2434, Brisbane, Qld 4001, Australia
[7] Nanjing Univ, Sch Atmospher Sci, Joint Int Res Lab Atmospher & Earth Syst Sci, Nanjing 210023, Jiangsu, Peoples R China
[8] Univ Helsinki, Dept Phys, Helsinki 00014, Finland
[9] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China
[10] Chinese Acad Meteorol Sci, CMA, Inst Atmospher Composit, Key Lab Atmospher Chem, Beijing 100081, Peoples R China
基金
中国国家自然科学基金;
关键词
PM2.5; Metropolitan regions; Chemical speciation; Control policies; China; YANGTZE-RIVER DELTA; EXTRACTABLE ORGANIC-COMPOUNDS; NUMBER SIZE DISTRIBUTIONS; PARTICLE FORMATION; LONG-TERM; SOURCE APPORTIONMENT; AIR-QUALITY; SEASONAL-VARIATION; HAZE POLLUTION; CHEMICAL-CHARACTERIZATION;
D O I
10.1016/j.scitotenv.2017.01.027
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
China is one of the regions with highest PM(2.5)concentration in the world. In this study, we review the spatio-temporal distribution of PM2.5 mass concentration and components in China and the effect of control measures on PM2.5 concentrations. Annual averaged PM2.5 concentrations in Central-Eastern China reached over 100 mu g m(-3), in some regions even over 150 mu g m(-3). In 2013, only 4.1% of the cities attained the annual average standard of 35 mu g m(-3). Aitken mode particles tend to dominate the total particle number concentration. Depending on the location and time of the year, new particle formation (NPF) has been observed to take place between about 10 and 60% of the days. In most locations, NPF was less frequent at high PM mass loadings. The secondary inorganic particles (i.e., sulfate, nitrate and ammonium) ranked the highest fraction among the PM2.5 species, followed by organic matters (OM), crustal species and element carbon (EC), which accounted for 6-50%, 15-51%, 5-41% and 2-12% of PM2.5, respectively. In response to serious particulate matter pollution, China has taken aggressive steps to improve air quality in the last decade. As a result, the national emissions of primary PM2.5, sulfur dioxide (SO2), and nitrogen oxides (NOx) have been decreasing since 2005, 2006, and 2011, respectively. The emission control policies implemented in the last decade could result in noticeable reduction in PM2,(5)concentrations, contributing to the decreasing PM2.5 trends observed in Beijing, Shanghai, and Guangzhou. However, the control policies issued before 2010 are insufficient to improve PM2.5 air quality notably in future. An optimal mix of energy-saving and end-of-pipe control measures should be implemented, more ambitious control policies for NMVOC and NH3 should be enforced, and special control measures in winter should be applied. 40-70% emissions should be cut off to attain PM2.5 standard. (C) 2017 Elsevier B.V.All rights reserved.
引用
收藏
页码:426 / 447
页数:22
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