Role of the Dipolar Interaction on the Macroscopic State of Magnetic Nanoparticle Systems: A Monte Carlo Study

被引:6
作者
Baldomir, D. [1 ,2 ]
Serantes, D. [1 ,2 ]
Pereiro, M. [1 ,2 ]
Botana, J. [1 ,2 ]
Arias, J. E. [1 ]
Masunaga, S. H. [2 ]
Rivas, J. [2 ]
机构
[1] Univ Santiago de Compostela, Inst Invest Tecnolox, E-15782 Santiago De Compostela, Galiza, Spain
[2] Univ Santiago de Compostela, Dept Fis Aplicada, E-15782 Santiago De Compostela, Galiza, Spain
关键词
Magnetic Nanoparticles; Monte Carlo Simulation; Magnetic Dipolar Interaction; ANISOTROPY;
D O I
10.1166/jnn.2010.1439
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We have performed Monte Carlo simulations to treat the effect of the dipolar interaction in assemblies of superparamagnetic nanoparticles. Our simulations reproduce correctly the increase of the blocking temperature (T-B) as the concentration increases, as observed experimentally. Interestingly, we have observed a progressive displacement of the M-2 versus H/M isotherms (Arrott plots) from the origin as the concentration of nanoparticles increases. Moreover, the curvature of the isotherms at T > T-B changes from positive to negative slope at high sample concentrations, resembling the shape of a first order phase transition. These results are surprisingly similar to that found in a conventional magnetic phase transition under the effect of a random anisotropy or a random field.
引用
收藏
页码:2717 / 2721
页数:5
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