Manganese-based catalysts supported on titania for the oxidation of nitric oxide

被引:0
作者
Li, Hua [1 ]
Tang, Xiaolong [1 ]
Yi, Honghong [1 ]
Yu, Lili [1 ]
机构
[1] Kunming Univ Sci &Technol, Kunming, Peoples R China
来源
2009 ASIA-PACIFIC POWER AND ENERGY ENGINEERING CONFERENCE (APPEEC), VOLS 1-7 | 2009年
关键词
NOx; NO oxidation; Manganese; TiO2;
D O I
暂无
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Manganese-based catalysts supported on TiO2 were studied for the oxidation of NO to NO2 in excess oxygen to remove NO from flue gas. Catalysts were prepared by incipient impregnation, excessive dipping and ultrasonic improved impregnation. The effects of precursor, manganese loadings, preparation method of catalysts and calcination temperature of catalysts on NO oxidation were investigated in details. Mn/TiO2-10% catalysts made from Mn(NO3)(2) and prepared by excessive dipping had the highest NO oxidation. More than 60% NO conversion was obtained at 200 degrees C under the condition of 500 ppm NO, 3% O-2 and the balance N-2, GHSV=19,200 h(-1).
引用
收藏
页码:2525 / 2528
页数:4
相关论文
共 9 条
[1]   Catalytic oxidation of nitrogen monoxide over Pt/SiO2 [J].
Després, J ;
Elsener, M ;
Koebel, M ;
Kröcher, O ;
Schnyder, B ;
Wokaun, A .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2004, 50 (02) :73-82
[2]  
MATTHEW M, 2007, J CATAL, P356
[3]   The influence of Pt oxide formation and Pt dispersion on the reactions NO2⇆NO+1/2 O2 over Pt/Al2O3 and Pt/BaO/Al2O3 [J].
Olsson, L ;
Fridell, E .
JOURNAL OF CATALYSIS, 2002, 210 (02) :340-353
[4]   MnOx-CeO2 mixed oxides prepared by co-precipitation for selective catalytic reduction of NO with NH3 at low temperatures [J].
Qi, GS ;
Yang, RT ;
Chang, R .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2004, 51 (02) :93-106
[5]   NO oxidation over supported Pt: Impact of precursor, support, loading, and processing conditions evaluated via high throughput experimentation [J].
Schmitz, P. J. ;
Kudla, R. J. ;
Drews, A. R. ;
Chen, A. E. ;
Lowe-Ma, C. K. ;
McCabe, R. W. ;
Schneider, W. F. ;
Goralski, C. T., Jr. .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2006, 67 (3-4) :246-256
[6]   Low temperature selective catalytic reduction of NOx with NH3 over amorphous MnOx catalysts prepared by three methods [J].
Tang, Xiaolong ;
Hao, Jiming ;
Xu, Wenguo ;
Li, Junhua .
CATALYSIS COMMUNICATIONS, 2007, 8 (03) :329-334
[7]  
TANG XL, 2007, CATAL TODAY, P406
[8]   Effect of filler types and calcination temperature on the microstructure and the nitric oxide photocatalytic activity of composite titanium dioxide films [J].
Wang, Haiqiang ;
Wu, Zhongbiao ;
Liu, Yue .
JOURNAL OF HAZARDOUS MATERIALS, 2009, 164 (2-3) :600-608
[9]   Roles of supports, Pt loading and Pt dispersion in the oxidation of NO to NO2 and of SO2 to SO3 [J].
Xue, E ;
Seshan, K ;
Ross, JRH .
APPLIED CATALYSIS B-ENVIRONMENTAL, 1996, 11 (01) :65-79