Risks related to heavy metal pollution in urban construction dust fall of fast-developing Chinese cities

被引:54
作者
Yang, Shaochen [1 ]
Liu, Jinling [1 ]
Bi, Xiangyang [1 ]
Ning, Yongqiang [1 ]
Qiao, Shengying [1 ]
Yu, Qianqian [1 ]
Zhang, Jie [2 ]
机构
[1] China Univ Geosci, Sch Earth Sci, Hubei Key Lab Crit Zone Evolut, Wuhan 430074, Peoples R China
[2] China Univ Geosci, Inst Math Geol & Remote Sensing, Wuhan 430074, Peoples R China
基金
中国国家自然科学基金;
关键词
Urban construction; Dust fall; Heavy metal; Risk assessment; HEALTH-RISK; AIR-POLLUTION; SOURCE APPORTIONMENT; HUMAN EXPOSURE; TRACE-METALS; STREET DUST; ROAD DUST; SOURCE IDENTIFICATION; FUGITIVE DUST; PM2.5;
D O I
10.1016/j.ecoenv.2020.110628
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Urban construction is a major contributor to air pollution, but few studies have examined heavy metal pollution in urban areas caused by construction dust fall. We measured the concentrations of Cr, Ni, Cu, Zn, Pb, Cd, and Hg and particle size distribution in dust fall from various construction activities in seven fast-developing cities in China and conducted a health risk assessment. Mean metal concentrations in construction dust fall were on the order of Zn (246.3 mg/kg) > Cr (94.2 mg/kg) > Pb (56.5 mg/kg) > Cu (53.6 mg/kg) > Ni (22.8 mg/kg) > Cd (0.68 mg/kg) > Hg (0.08 mg/kg). Cu and Zn were positively correlated in areas of subway and building construction, and Pb and Cd were positively correlated in areas of road construction, likely because of the materials specific to these activities. Enrichment factors for heavy metals at all sampling sites were on the order of Cd (10.4) > Zn (6.37) > Cu (4.25) > Pb (3.84) > Hg (2.41) > Cr (2.02) > Ni (1.32). The enrichment factors for all metals except Zn indicated that heavy metal pollution was highest in road construction, followed by building and subway construction. Non-carcinogenic risks to children (hazard index> 1) were 1.01-1.08 in four of the seven sampling sites, indicating possible risk from deposition of construction dust fall. In contrast, the hazard index for adults was < 1 at the seven cities and total carcinogenic risks (< 1x10(-6)) were at acceptable levels. An integrated ecological risk assessment demonstrated that heavy metal particles in construction dust fall in two of the cities (Shijiazhuang and Qingdao) were likely to be suspended in the atmosphere. Our study of heavy metal pollution in construction dust fall provides data on ecological and human health impacts and suggests that extensive measures are required to control construction dust fall in China.
引用
收藏
页数:9
相关论文
共 56 条
[1]  
[Anonymous], 2002, SHORT TERM METHODS E, P1
[2]  
[Anonymous], [No title captured]
[3]  
[Anonymous], [No title captured]
[4]  
[Anonymous], [No title captured]
[5]  
[Anonymous], 2013, China Statistical Yearbook 2013
[6]  
[Anonymous], [No title captured]
[7]   In vitro bioaccessibility of lead in surface dust and implications for human exposure: A comparative study between industrial area and urban district [J].
Bi, Xiangyang ;
Li, Zhonggen ;
Sun, Guangyi ;
Liu, Jinling ;
Han, Zhixuan .
JOURNAL OF HAZARDOUS MATERIALS, 2015, 297 :191-197
[8]   A review of the distribution of particulate trace elements in urban terrestrial environments and its application to considerations of risk [J].
Charlesworth, S. ;
De Miguel, E. ;
Ordonez, A. .
ENVIRONMENTAL GEOCHEMISTRY AND HEALTH, 2011, 33 (02) :103-123
[9]   Occupational health risk assessment based on actual dust exposure in a tunnel construction adopting roadheader in Chongqing, China [J].
Chen, Xiaofeng ;
Guo, Chun ;
Song, Junxiu ;
Wang, Xin ;
Cheng, Jianghao .
BUILDING AND ENVIRONMENT, 2019, 165
[10]  
[成杭新 Cheng Hangxin], 2014, [地学前缘, Earth Science Frontiers], V21, P265