Deposition of Pt on the stable nanotubular TiO2 and its photocatalytic performance

被引:52
作者
An, Huiqin [1 ]
Zhou, Jian [1 ]
Li, Junxia [1 ]
Zhu, Baolin [1 ]
Wang, Shurong [1 ]
Zhang, Shoumin [1 ]
Wu, Shihua [1 ]
Huang, Weiping [1 ]
机构
[1] Nankai Univ, Dept Chem, Tianjin 300071, Peoples R China
基金
中国国家自然科学基金;
关键词
TiO2; nanotubes; Platinum; Stability; Photocatalytic activity; VISIBLE-LIGHT IRRADIATION; TITANATE; PLATINUM; PHOTODEGRADATION; NANOPARTICLES; OXIDATION; BEHAVIOR; CO;
D O I
10.1016/j.catcom.2009.09.020
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The stable nanotubular TiO2 prepared by treating hydrogen titanate nanotubes with sol containing titanium is used as support, and platinum nanoparticles are loaded on the support via photodeposition process. The obtained Rt/TiO2 nanotubes are characterized with transmission electron microscopy, X-ray diffraction, UV-vis absorption spectroscopy and nitrogen adsorption. The photocatalytic performance is evaluated by the photocatalytic degradation rates of methyl orange under UV light irradiation. The results show that the nanotubular structure of support is intact during photodeposition and the Pt/TiO2 nanotubes exhibit higher photocatalytic activity. Crown Copyright (C) 2009 Published by Elsevier B.V. All rights reserved.
引用
收藏
页码:175 / 179
页数:5
相关论文
共 31 条
[1]   Synthesis and Characterization of Thermally Stable Nanotubular TiO2 and Its Photocatalytic Activity [J].
An, Huiqin ;
Zhu, Baolin ;
Li, Junxia ;
Zhou, Jian ;
Wang, Shurong ;
Zhang, Shoumin ;
Wu, Shihua ;
Huang, Weiping .
JOURNAL OF PHYSICAL CHEMISTRY C, 2008, 112 (48) :18772-18775
[2]   Protonated titanates and TiO2 nanostructured materials:: Synthesis, properties, and applications [J].
Bavykin, Dmitry V. ;
Friedrich, Jens M. ;
Walsh, Frank C. .
ADVANCED MATERIALS, 2006, 18 (21) :2807-2824
[3]   Effect Of Pt/TiO2 characteristics on temporal behavior of o-cresol decomposition by visible light-induced photocatalysis [J].
Chen, Hua-Wei ;
Ku, Young ;
Kuo, Yu-Lin .
WATER RESEARCH, 2007, 41 (10) :2069-2078
[4]   Structure and applications of titanate and related nanostructures [J].
Chen, Q. ;
Peng, L-M. .
INTERNATIONAL JOURNAL OF NANOTECHNOLOGY, 2007, 4 (1-2) :44-65
[5]   Titanium dioxide nanomaterials: Synthesis, properties, modifications, and applications [J].
Chen, Xiaobo ;
Mao, Samuel S. .
CHEMICAL REVIEWS, 2007, 107 (07) :2891-2959
[6]   Synthesis, Characterization of Fe-doped TiO2 Nanotubes with High Photocatalytic Activity [J].
Deng, Lixue ;
Wang, Shurong ;
Liu, Daying ;
Zhu, Baolin ;
Huang, Weiping ;
Wu, Shihua ;
Zhang, Shoumin .
CATALYSIS LETTERS, 2009, 129 (3-4) :513-518
[7]   The surface science of titanium dioxide [J].
Diebold, U .
SURFACE SCIENCE REPORTS, 2003, 48 (5-8) :53-229
[8]  
Fujishima A., 2000, J. Photochem. Photobiol. C: Photochem. Rev., V1, P1, DOI [10.1016/S1389-5567(00)00002-2, DOI 10.1016/S1389-5567(00)00002-2]
[9]   Highly enhanced photocatalytic oxidation of CO on titania deposited with Pt nanoparticles: kinetics and mechanism [J].
Hwang, S ;
Lee, MC ;
Choi, W .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2003, 46 (01) :49-63
[10]   Formation of titanium oxide nanotube [J].
Kasuga, T ;
Hiramatsu, M ;
Hoson, A ;
Sekino, T ;
Niihara, K .
LANGMUIR, 1998, 14 (12) :3160-3163