Frequency domain quantum optimal control under multiple constraints

被引：34

作者：

Shu, Chuan-Cun ^{[1
,2
]}

Ho, Tak-San ^{[1
]}

Xing, Xi ^{[1
]}

Rabitz, Herschel ^{[1
]}

机构：

[1] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA

[2] Univ New S Wales, Australian Def Force Acad, Sch Engn & Informat Technol, Canberra, ACT 2600, Australia

来源：

PHYSICAL REVIEW A | 2016年 / 93卷 / 03期

基金：

美国国家科学基金会;

关键词：

DYNAMICS;

D O I：

10.1103/PhysRevA.93.033417

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

Optimal control of quantum systems with complex constrained external fields is one of the longstanding theoretical and numerical challenges at the frontier of quantum control research. Here, we present a theoretical method that can be utilized to optimize the control fields subject to multiple constraints while guaranteeing monotonic convergence towards desired physical objectives. This optimization method is formulated in the frequency domain in line with the current ultrafast pulse shaping technique, providing the possibility for performing quantum optimal control simulations and experiments in a unified fashion. For illustrations, this method is successfully employed to perform multiple constraint spectral-phase-only optimization for maximizing resonant multiphoton transitions with desired pulses.

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页数：5

相关论文

共 49 条

[1] Optimal Control of Open Quantum Systems Applied to the Photochemistry of Surfaces [J].

Asplund, Erik ;

Kluener, Thorsten .

PHYSICAL REVIEW LETTERS, 2011, 106 (14)

[2] Control of chemical reactions by feedback-optimized phase-shaped femtosecond laser pulses [J].

Assion, A ;

Baumert, T ;

Bergt, M ;

Brixner, T ;

Kiefer, B ;

Seyfried, V ;

Strehle, M ;

Gerber, G .

SCIENCE, 1998, 282 (5390) :919-922

[3]

Barmes I, 2013, NAT PHOTONICS, V7, P38, DOI [10.1038/NPHOTON.2012.299, 10.1038/nphoton.2012.299]

[4] Optimal local control of coherent dynamics in custom-made nanostructures [J].

Blasi, Thomas ;

Borunda, Mario F. ;

Rasanen, Esa ;

Heller, Eric J. .

PHYSICAL REVIEW B, 2013, 87 (24)

[5] Control of quantum phenomena: past, present and future [J].

Brif, Constantin ;

Chakrabarti, Raj ;

Rabitz, Herschel .

NEW JOURNAL OF PHYSICS, 2010, 12

[6] Plasmonic antennas as design elements for coherent ultrafast nanophotonics [J].

Brinks, Daan ;

Castro-Lopez, Marta ;

Hildner, Richard ;

van Hulst, Niek F. .

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2013, 110 (46) :18386-18390

[7] Photoselective adaptive femtosecond quantum control in the liquid phase [J].

Brixner, T ;

Damrauer, NH ;

Niklaus, P ;

Gerber, G .

NATURE, 2001, 414 (6859) :57-60

[8] Understanding learning control of molecular fragmentation [J].

Cardoza, D ;

Baertschy, M ;

Weinacht, T .

CHEMICAL PHYSICS LETTERS, 2005, 411 (4-6) :311-315

[9] Controlling the Dynamics of Many-Electron Systems from First Principles: A Combination of Optimal Control and Time-Dependent Density-Functional Theory [J].

Castro, A. ;

Werschnik, J. ;

Gross, E. K. U. .

PHYSICAL REVIEW LETTERS, 2012, 109 (15)

[10] Optimal Quantum Control of Multimode Couplings between Trapped Ion Qubits for Scalable Entanglement [J].

Choi, T. ;

Debnath, S. ;

Manning, T. A. ;

Figgatt, C. ;

Gong, Z. -X. ;

Duan, L. -M. ;

Monroe, C. .

PHYSICAL REVIEW LETTERS, 2014, 112 (19)

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