A strategy for scaling up the Fischer-Tropsch bubble column slurry reactor

被引:14
作者
Krishna, R [1 ]
van Baten, JM [1 ]
机构
[1] Univ Amsterdam, Dept Chem Engn, NL-1018 WV Amsterdam, Netherlands
关键词
gas holdup; bubble columns; scale effects; computational fluid dynamics; liquid circulations; concentrated slurries;
D O I
10.1023/B:TOCA.0000012984.86721.bc
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
For successful scale-up of the bubble column slurry reactor for Fischer - Tropsch synthesis, we need to have proper description of hydrodynamics and transport phenomena ( gas and liquid holdups, liquid-phase residence time distribution, gas - liquid mass transfer, heat transfer to cooling tubes) as a function of reactor scale ( column diameter and height) and operating conditions ( superficial gas velocity, system pressure, slurry concentration,...). We discuss and develop a scale-up strategy using computational fluid dynamics, with a minimum amount of experimental input from hydrodynamic studies carried out on a relatively small scale.
引用
收藏
页码:21 / 28
页数:8
相关论文
共 25 条
[11]  
Krishna R, 2001, CHEM ENG TECHNOL, V24, P451, DOI 10.1002/1521-4125(200105)24:5<451::AID-CEAT451>3.0.CO
[12]  
2-8
[13]   Design and scale up of a bubble column slurry reactor for Fischer-Tropsch synthesis [J].
Krishna, R ;
van Baten, JM ;
Urseanu, MI ;
Ellenberger, J .
CHEMICAL ENGINEERING SCIENCE, 2001, 56 (02) :537-545
[14]   A scale-up strategy for a commercial scale bubble column slurry reactor for Fischer-Tropsch synthesis [J].
Krishna, R .
OIL & GAS SCIENCE AND TECHNOLOGY-REVUE D IFP ENERGIES NOUVELLES, 2000, 55 (04) :359-393
[15]   Gas holdup and mass transfer in bubble column reactors operated at elevated pressure [J].
Letzel, HM ;
Schouten, JC ;
Krishna, R ;
van den Bleek, CM .
CHEMICAL ENGINEERING SCIENCE, 1999, 54 (13-14) :2237-2246
[16]   Influence of elevated pressure on the stability of bubbly flows [J].
Letzel, HM ;
Schouten, JC ;
vandenBleek, CM ;
Krishna, R .
CHEMICAL ENGINEERING SCIENCE, 1997, 52 (21-22) :3733-3739
[17]   Characterization of regimes and regime transitions in bubble columns by chaos analysis of pressure signals [J].
Letzel, HM ;
Schouten, JC ;
Krishna, R ;
van den Bleek, CM .
CHEMICAL ENGINEERING SCIENCE, 1997, 52 (24) :4447-4459
[18]   Effect of gas density on large-bubble holdup in bubble column reactors [J].
Letzel, MH .
AICHE JOURNAL, 1998, 44 (10) :2333-2336
[19]   Modelling of a bubble column slurry reactor for Fischer-Tropsch synthesis [J].
Maretto, C ;
Krishna, R .
CATALYSIS TODAY, 1999, 52 (2-3) :279-289
[20]   Dynamic simulation of bubbly flow in bubble columns [J].
Pan, Y ;
Dudukovic, MP ;
Chang, M .
CHEMICAL ENGINEERING SCIENCE, 1999, 54 (13-14) :2481-2489