Ultrafast vibrational energy transfer between surface and bulk water at the air-water interface

被引：100
|
作者：
Smits, Marc
Ghosh, Avishek
Sterrer, Martin
Muller, Michiel
Bonn, Mischa
机构：
[1] FOM, Inst Atom & Mol Phys, NL-1098 SJ Amsterdam, Netherlands
[2] Leiden Univ, Leiden Inst Chem, NL-2300 RA Leiden, Netherlands
[3] Max Planck Gesell, Fritz Haber Inst, D-14195 Berlin, Germany
[4] Univ Amsterdam, Swammerdam Inst Life Sci, NL-1090 GB Amsterdam, Netherlands
来源：
PHYSICAL REVIEW LETTERS | 2007年 / 98卷 / 09期
关键词：
D O I：
10.1103/PhysRevLett.98.098302
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
We report a femtosecond time-resolved study of water at the neat water-air interface. The O-H stretch vibrational lifetime of hydrogen-bonded interfacial water is measured using surface-specific 4th-order nonlinear optical spectroscopy with femtosecond infrared pulses. The vibrational lifetime in the frequency range of 3200 to 3500 cm(-1) is found to closely resemble that of bulk water, indicating ultrafast exchange of vibrational energy between surface water molecules and those in the bulk.
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页数：4
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