Sb doped SnO2-decorated porous g-C3N4 nanosheet heterostructures with enhanced photocatalytic activities under visible light irradiation

被引:134
作者
Yang, Liuqing [1 ,2 ]
Huang, Jianfeng [1 ]
Shi, Li [2 ]
Cao, Liyun [1 ]
Liu, Huimin [2 ]
Liu, Yanyu [3 ]
Li, Yunxiang [2 ]
Song, Hui [2 ]
Jie, Yanni [1 ]
Ye, Jinhua [2 ,4 ,5 ]
机构
[1] Shaanxi Univ Sci & Technol, Sch Mat Sci & Engn, Xian 710021, Shaanxi, Peoples R China
[2] NIMS, Int Ctr Mat Nanoarchitect WPI MANA, 1-1 Namiki, Tsukuba, Ibaraki 3050044, Japan
[3] Tianjin Univ, Fac Sci, Tianjin Key Lab Low Dimens Mat Phys & Preparing T, Dept Appl Phys, Tianjin 300072, Peoples R China
[4] Tianjin Univ, Sch Mat Sci & Engn, TU NIMS Int Collaborat Lab, 92 Weijin Rd, Tianjin 300072, Peoples R China
[5] Collaborat Innovat Ctr Chem Sci & Engn Tianjin, Tianjin 300072, Peoples R China
基金
中国国家自然科学基金;
关键词
g-C3N4; Sb doped SnO2; Heterostructure; Photocatalytic CO2 reduction; Photocatalytic IPA oxidation; GRAPHITIC CARBON NITRIDE; CHARGE SEPARATION EFFICIENCY; HYDROGEN-EVOLUTION; FENTON REACTION; COMPOSITE; SURFACE; OXIDE; CO2; REDUCTION; HETEROJUNCTION;
D O I
10.1016/j.apcatb.2017.09.041
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A novel Sb doped SnO2 decorated porous g-C3N4 nanosheet composite photocatalyst, which can be applied in photocatalytic reactions for CO2 reduction and gaseous iso-isopropanol (IPA) oxidation under visible light irradiation, is designed and synthesized. Results demonstrate that the intimate interfacial contact and heterojunction interaction between g-C3N4 and Sb doped SnO2 can significantly boost the photocatalytic efficiencies compared with individual g-C3N4 and Sb doped SnO2 due to the effective separation of photo-generated charge carriers.
引用
收藏
页码:670 / 680
页数:11
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