Photocatalytic activity of novel Bi2WO6/CNFs composite synthesized via two distinct solvothermal steps

被引:6
作者
Wang, Yong [1 ,2 ]
Sunarso, Jaka [3 ]
Chen, Guihua [1 ]
Zhao, Songlin [1 ]
Liu, Zhenzhong [4 ]
Wei, Yeyun [1 ]
机构
[1] Taizhou Univ, Sch Pharmaceut & Chem Engn, Jiaojiang 318000, Peoples R China
[2] Nanjing Tech Univ, Coll Chem & Chem Engn, Nanjing 210009, Jiangsu, Peoples R China
[3] Swinburne Univ Technol, Fac Engn Comp & Sci, Jalan Simpang Tiga, Kuching 93350, Sarawak, Malaysia
[4] Res Inst Zhejiang Univ, Taizhou 318000, Jiaojiang, Peoples R China
关键词
Carbon materials; Semiconductors; Nanocomposites; Photocatalysis; VISIBLE-LIGHT; CARBON NANOFIBERS; ACTIVATED CARBON; PROPERTY;
D O I
10.1016/j.matlet.2017.03.144
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Here, we report the synthesis of Bi2WO6/carbon nanofibers (CNFs) composite with a unique surface morphology, i.e., its surface was fully decorated with crisscrossed Bi2WO6 nanoplates, via two solvothermal steps using ethanol and ethylene glycol as solvent medium in the first and the second step, respectively. Such composite demonstrated significant enhancement for photocatalytic activity relative to Bi2WO6 and mechanical mixture of Bi2WO6 with CNFs, leading to the highest degradation rate of methyl orange (MO) using the composite catalyst under visible light irradiation where up to 92% of MO could be degraded within 360 min period. We attribute this to an efficient separation of photogenerated electrons and holes due to the formation of heterostructure between Bi2WO6 and CNFs in the composite. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:102 / 105
页数:4
相关论文
共 12 条
[1]   BiOCl nanosheets immobilized on electrospun polyacrylonitrile nanofibers with high photocatalytic activity and reusable property [J].
Chou, Yuechen ;
Shao, Changlu ;
Li, Xinghua ;
Su, Chunyan ;
Xu, Hongchuan ;
Zhang, Mingyi ;
Zhang, Peng ;
Zhang, Xin ;
Liu, Yichun .
APPLIED SURFACE SCIENCE, 2013, 285 :509-516
[2]   CdS loaded on coal based activated carbon nanofibers with enhanced photocatalytic property [J].
Guo, Jixi ;
Guo, Mingxi ;
Jia, Dianzeng ;
Song, Xianli ;
Tong, Fenglian .
CHEMICAL PHYSICS LETTERS, 2016, 659 :66-69
[3]   Enhanced photocatalytic activity of ZnO microflower arrays synthesized by one-step etching approach [J].
Li, Xiuyan ;
Wang, Jian ;
Yang, Jinghai ;
Lang, Jihui ;
Wei, Maobin ;
Meng, Xiangwei ;
Lu, Shiquan ;
Sui, Yingrui .
JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL, 2013, 378 :1-6
[4]   High Photocatalytic Activity of ZnO-Carbon Nanofiber Heteroarchitectures [J].
Mu, Jingbo ;
Shao, Changlu ;
Guo, Zengcai ;
Zhang, Zhenyi ;
Zhang, Mingyi ;
Zhang, Peng ;
Chen, Bin ;
Liu, Yichun .
ACS APPLIED MATERIALS & INTERFACES, 2011, 3 (02) :590-596
[5]   Role of activated carbon on the increased photocatalytic activity of AC/Bi2WO6 coupled materials [J].
Murcia-Lopez, S. ;
Navio, J. A. ;
Hidalgo, M. C. .
APPLIED CATALYSIS A-GENERAL, 2013, 466 :51-59
[6]   Synthesis and photocatalytic activities of CdS/TiO2 nanoparticles supported on carbon nanofibers for high efficient adsorption and simultaneous decomposition of organic dyes [J].
Pant, Bishweshwar ;
Barakat, Nasser A. M. ;
Pant, Hem Raj ;
Park, Mira ;
Saud, Prem Singh ;
Kim, Jong-Wan ;
Kim, Hak-Yong .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2014, 434 :159-166
[7]   Bi2WO6 nanocrystals with high photocatalytic activities under visible light [J].
Shang, Meng ;
Wang, Wenzhong ;
Sun, Songmei ;
Zhou, Lin ;
Zhang, Ling .
JOURNAL OF PHYSICAL CHEMISTRY C, 2008, 112 (28) :10407-10411
[8]   Novel synthesis of bismuth tungstate hollow nanospheres in water-ethanol mixed solvent [J].
Wu, Daxiong ;
Zhu, Haitao ;
Zhang, Canying ;
Chen, Lei .
CHEMICAL COMMUNICATIONS, 2010, 46 (38) :7250-7252
[9]   Biomimetic Bi2WO6 with hierarchical structures from butterfly wings for visible light absorption [J].
Yao, Fan ;
Yang, Qingqing ;
Yin, Chao ;
Zhu, Shenmin ;
Zhang, Di ;
Moon, Won-Jin ;
Kim, Yang-Soo .
MATERIALS LETTERS, 2012, 77 :21-24
[10]   Mesoporous Fe2O3-doped TiO2 nanostructured fibers with higher photocatalytic activity [J].
Zhan, Sihui ;
Yang, Jiangyao ;
Liu, Yu ;
Wang, Nan ;
Dai, Jingjing ;
Yu, Hongbing ;
Gao, Xichao ;
Li, Yi .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2011, 355 (02) :328-333