Time-Domain Infrared-Visible-Visible Sum-Frequency Generation for Surface Vibrational Spectroscopy

被引：6
|
作者：
Nomoto, Tomonori [1 ]
Onishi, Hiroshi [2 ]
机构：
[1] Kobe Univ, Mol Photosci Res Ctr, Nada Ku, Kobe, Hyogo 6578501, Japan
[2] Kobe Univ, Dept Chem, Grad Sch Sci, Nada Ku, Kobe, Hyogo 6578501, Japan
来源：
JOURNAL OF PHYSICAL CHEMISTRY C | 2009年 / 113卷 / 52期
关键词：
2ND-HARMONIC GENERATION; RAMAN-SPECTROSCOPY; RUTILE; TIO2; SCATTERING; RADIATION; CONSTANTS; DYNAMICS; MODES; FIELD;
D O I：
10.1021/jp908308t
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
We propose a new surface-sensitive, time-domain measurement of low-frequency vibrational coherence. A transverse optical phonon was coherently excited at 180 cm(-1) on a TiO(2) (110) wafer by femtosecond terahertz pulses of the far-infrared region. The probability of second harmonic generation was modulated by the coherent lattice vibrations and probed using visible light pulses. The observable depth was limited as small as 3 nm by tuning the wavelength of the second harmonic light to be resonant with the electronic absorption of TiO(2).
引用
收藏
页码：21467 / 21470
页数：4
相关论文
共 50 条
  • [21] Sum-frequency spectroscopy on bulk and surface phonons of noncentrosymmetric crystals
    Liu, Wei-Tao
    Shen, Y. R.
    ANNALEN DER PHYSIK, 2011, 523 (1-2) : 101 - 106
  • [22] General Normalizing Approach for Broadband Infrared Sum-Frequency Generation Spectroscopy via a Transmitted Signal in α-Quartz
    Zeng, Wei-Wang
    Luo, Ting
    Zhou, Chuanyao
    Ren, Zefeng
    JOURNAL OF PHYSICAL CHEMISTRY C, 2024, 128 (09) : 4018 - 4023
  • [23] A Theoretical Investigation of Surface-enhanced Sum-frequency Generation
    Yeh, Y. L.
    Lei, J.
    Chen, S. Y.
    Chang, A. H. H.
    Lin, C. K.
    He, R. X.
    Lin, S. H.
    JOURNAL OF THE CHINESE CHEMICAL SOCIETY, 2016, 63 (01) : 136 - 144
  • [24] Effect of deuteration on a phosphatidylcholine lipid monolayer structure: New insights from vibrational sum-frequency generation spectroscopy
    Navakauskas, Edvinas
    Niaura, Gediminas
    Strazdaite, Simona
    COLLOIDS AND SURFACES B-BIOINTERFACES, 2022, 220
  • [25] Sequential wavelength tuning:: Dynamics at interfaces investigated by vibrational sum-frequency spectroscopy
    Schrodle, Simon
    Richmond, Geraldine L.
    APPLIED SPECTROSCOPY, 2008, 62 (04) : 389 - 393
  • [26] Assessing the Impact of Solvent Selection on Vibrational Sum-Frequency Scattering Spectroscopy Experiments
    Carpenter, Andrew P.
    Christoffersen, Evan L.
    Mapile, Ashley N.
    Richmond, Geraldine L.
    JOURNAL OF PHYSICAL CHEMISTRY B, 2021, 125 (12) : 3216 - 3229
  • [27] A new approach to vibrational sum frequency generation spectroscopy using near infrared pulse shaping
    Chowdhury, Azhad U.
    Watson, Brianna R.
    Ma, Ying-Zhong
    Sacci, Robert L.
    Lutterman, Daniel A.
    Calhoun, Tessa R.
    Doughty, Benjamin
    REVIEW OF SCIENTIFIC INSTRUMENTS, 2019, 90 (03)
  • [28] Time-domain spectroscopy in the mid-infrared
    Lanin, A. A.
    Voronin, A. A.
    Fedotov, A. B.
    Zheltikov, A. M.
    SCIENTIFIC REPORTS, 2014, 4
  • [29] Vibrational Sum-Frequency Generation Study of Morpholine at Air-Liquid and Air-Solution Interfaces
    SenGupta, Sumana
    Saha, Ankur
    Kumar, Awadhesh
    Naik, P. D.
    JOURNAL OF PHYSICAL CHEMISTRY C, 2016, 120 (36) : 20132 - 20141
  • [30] Tutorials in vibrational sum frequency generation spectroscopy. III. Collecting, processing, and analyzing vibrational sum frequency generation spectra
    Pickering, James D. D.
    Bregnhoj, Mikkel
    Rasmussen, Mette H. H.
    Strunge, Kris
    Weidner, Tobias
    BIOINTERPHASES, 2022, 17 (04)
12345