Femtosecond carrier dynamics and saturable absorption in graphene suspensions

被引:192
作者
Kumar, Sunil [1 ,2 ]
Anija, M. [1 ,2 ]
Kamaraju, N. [1 ,2 ]
Vasu, K. S. [1 ]
Subrahmanyam, K. S. [3 ,4 ]
Sood, A. K. [1 ,2 ,3 ,4 ]
Rao, C. N. R. [1 ,3 ,4 ]
机构
[1] Indian Inst Sci, Dept Phys, Bangalore 560012, Karnataka, India
[2] Indian Inst Sci, Ctr Ultrafast Laser Applicat, Bangalore 560012, Karnataka, India
[3] Jawaharlal Nehru Ctr Adv Sci Res, Chem & Phys Mat Unit, Bangalore 560064, Karnataka, India
[4] Jawaharlal Nehru Ctr Adv Sci Res, Int Ctr Mat Sci, Bangalore 560064, Karnataka, India
关键词
GRAPHITE; FILMS;
D O I
10.1063/1.3264964
中图分类号
O59 [应用物理学];
学科分类号
摘要
Nonlinear optical properties and carrier relaxation dynamics in graphene, suspended in three different solvents, are investigated using femtosecond (80 fs pulses) Z-scan and degenerate pump-probe spectroscopy at 790 nm. The results demonstrate saturable absorption property of graphene with a nonlinear absorption coefficient, beta of (similar to 2-9) x 10(-8) cm/W. Two distinct time scales associated with the relaxation of photoexcited carriers, a fast one in the range of 130-330 fs (related to carrier-carrier scattering) followed by it slower one in 3.5-4.9 ps range (associated with carrier-phonon scattering) are observed. (C) 2009 American Institute of Physics. [doi:10.1063/1.3264964]
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页数:3
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