Cesium lead halide perovskite quantum dot-based warm white light-emitting diodes with high color rendering index

被引:21
作者
Bi, Ke [1 ]
Wang, Dan [1 ]
Wang, Peng [1 ]
Duan, Bin [1 ]
Zhang, Tieqiang [1 ]
Wang, Yinghui [1 ]
Zhang, Hanzhuang [1 ]
Zhang, Yu [2 ,3 ]
机构
[1] Jilin Univ, Minist Educ, Key Lab Phys & Technol Adv Batteries, Femtosecond Laser Lab,Coll Phys, Changchun 130012, Peoples R China
[2] Jilin Univ, State Key Lab Integrated Optoelect, Changchun 130012, Peoples R China
[3] Jilin Univ, Coll Elect Sci & Engn, Changchun 130012, Peoples R China
基金
中国国家自然科学基金;
关键词
Perovskite; Quantum dots; White light-emitting diodes; PHOSPHORS; NANOCRYSTALS; EMISSION; EFFICIENT; CSPBX3; LEDS; LUMINESCENCE; FILMS;
D O I
10.1007/s11051-017-3862-2
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
White light-emitting diodes (WLEDs) were fabricated by employing a combination of a commercial yellow emission Ce3+-doped Y3Al5O12 (YAG:Ce)-based phosphor and all-inorganic perovskite quantum dots pumped with blue LED chip. Perovskite quantum dot solution was used as the color conversion layer with liquid-type structure. Red-emitting materials based on cesium lead halide (CsPb(X)(3)) perovskite quantum dots were introduced to generate WLEDs with high efficacy and high color rendering index through compensating the red emission of the YAG: Ce phosphor-based commercialized WLEDs. The experimental results suggested that the luminous efficiency and color rendering index of the as-prepared WLED device could reach up to 84.7 mu m/Wand 89, respectively. The characteristics of those devices including correlated color temperature (CCT), color rendering index (CRI), and color coordinates were observed under different forward currents. The as-fabricated warm WLEDs showed excellent color stability against the increasing current, while the color coordinates shifted slightly from (0.3837, 0.3635) at 20 mA to (0.3772, 0.3592) at 120 mA and color temperature tuned from 3803 to 3953 K.
引用
收藏
页数:8
相关论文
共 34 条
[1]   Tuning the Optical Properties of Cesium Lead Halide Perovskite Nanocrystals by Anion Exchange Reactions [J].
Akkerman, Quinten A. ;
D'Innocenzo, Valerio ;
Accornero, Sara ;
Scarpellini, Alice ;
Petrozza, Annamaria ;
Prato, Mirko ;
Manna, Liberato .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2015, 137 (32) :10276-10281
[2]   Temperature Quenching of Yellow Ce3+ Luminescence in YAG:Ce [J].
Bachmann, Volker ;
Ronda, Cees ;
Meijerink, Andries .
CHEMISTRY OF MATERIALS, 2009, 21 (10) :2077-2084
[3]   Efficient and tuneable photoluminescent boehmite hybrid nanoplates lacking metal activator centres for single-phase white LEDs [J].
Bai, Xue ;
Caputo, Gianvito ;
Hao, Zhendong ;
Freitas, Vania T. ;
Zhang, Jiahua ;
Longo, Ricardo L. ;
Malta, Oscar L. ;
Ferreira, Rute A. S. ;
Pinna, Nicola .
NATURE COMMUNICATIONS, 2014, 5
[4]   Stability of the Mn photoluminescence in bifunctional ZnS:0.05Mn nanoparticles [J].
Beltran-Huarac, Juan ;
Wang, Jingzhou ;
Tanaka, Hiroki ;
Jadwisienczak, Wojciech M. ;
Weiner, Brad R. ;
Morell, Gerardo .
JOURNAL OF APPLIED PHYSICS, 2013, 114 (05)
[5]   Red emissive CuInS2-based nanocrystals: a potential phosphor for warm white light-emitting diodes [J].
Chen, Bingkun ;
Zhou, Qingchao ;
Li, Junfei ;
Zhang, Feng ;
Liu, Ruibin ;
Zhong, Haizheng ;
Zou, Bingsuo .
OPTICS EXPRESS, 2013, 21 (08) :10105-10110
[6]   Color-Tuned Perovskite Films Prepared for Efficient Solar Cell Applications [J].
Cui, Dong ;
Yang, Zhou ;
Yang, Dong ;
Ren, Xiaodong ;
Liu, Yucheng ;
Wei, Qingbo ;
Fan, Haibo ;
Zeng, Jinghui ;
Liu, Shengzhong .
JOURNAL OF PHYSICAL CHEMISTRY C, 2016, 120 (01) :42-47
[7]   Mixed Iodide-Bromide Methylammonium Lead Perovskite-based Diodes for Light Emission and Photovoltaics [J].
Gil-Escrig, Lidon ;
Miquel-Sempere, Araceli ;
Sessolo, Michele ;
Bolink, Henk J. .
JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 2015, 6 (18) :3743-3748
[8]   Electronic band structure, phonons, and exciton binding energies of halide perovskites CsSnCl3, CsSnBr3, and CsSnI3 [J].
Huang, Ling-yi ;
Lambrecht, Walter R. L. .
PHYSICAL REVIEW B, 2013, 88 (16)
[9]   Preparation of a photo-degradation-resistant quantum dot-polymer composite plate for use in the fabrication of a high-stability white-light-emitting diode [J].
Jang, Eun-Pyo ;
Song, Woo-Seuk ;
Lee, Ki-Heon ;
Yang, Heesun .
NANOTECHNOLOGY, 2013, 24 (04)
[10]   White-Light-Emitting Diodes with Quantum Dot Color Converters for Display Backlights [J].
Jang, Eunjoo ;
Jun, Shinae ;
Jang, Hyosook ;
Llim, Jungeun ;
Kim, Byungki ;
Kim, Younghwan .
ADVANCED MATERIALS, 2010, 22 (28) :3076-3080