MXene-based rGO/Nb2CTx/Fe3O4 composite for high absorption of electromagnetic wave

被引:167
作者
Cui, Ce [1 ,2 ]
Guo, Ronghui [1 ,2 ]
Ren, Erhui [1 ,2 ]
Xiao, Hongyan [1 ,2 ]
Zhou, Mi [1 ,2 ]
Lai, Xiaoxu [1 ,2 ]
Qin, Qin [1 ,2 ]
Jiang, Shouxiang [3 ]
Qin, Wenfeng [4 ]
机构
[1] Sichuan Univ, Coll Biomass Sci & Engn, Chengdu 610065, Peoples R China
[2] Sichuan Univ, Minist Educt, Key Lab Leather Chemisty & Engn, Chengdu 610065, Sichuan, Peoples R China
[3] Hong Kong Polytech Univ, Inst Text & Clothing, Kowloon, Hong Kong 999077, Peoples R China
[4] Civil Aviat Flight Univ China, Aviat Engn Inst, Guanghan 618307, Peoples R China
基金
中国国家自然科学基金;
关键词
MXene; Hierarchical architecture; rGO/Nb2CTx/Fe3O4; composite; Electromagnetic wave absorption; MICROWAVE-ABSORPTION; HIERARCHICAL ARCHITECTURE; GRAPHENE; PERFORMANCE; HYBRID; NANOPARTICLES; NANOSHEETS; MICROSPHERES; FABRICATION; LIGHTWEIGHT;
D O I
10.1016/j.cej.2020.126626
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A rGO/Nb2CTx/Fe3O4 composite with a hierarchical architecture is prepared by integrating multilayered Nb2CTx, magnetic Fe3O4 nanoparticles and two-dimensional rGO sheets. The rGO/Nb(2)CTx/Fe3O4 composite shows superior absorption of electromagnetic wave with a minimum reflection loss (RLmin) of -59.17 dB at 11.8 GHz with an equal absorber thickness of 2.5 mm as well as a broad effective absorption bandwidth (EAB, RL <= 10 dB) of 6.8 GHz. The tunable EAB can be achieved at a frequency range of 8.5 to 18 GHz by modifying the thickness of the absorber from 1.5 to 3 mm. The excellent absorption capacity of electromagnetic wave is attributed to the synergetic effects between the multiple loss mechanisms of rGO/Nb2CTx/Fe3O4 and good impedance matching. The results provide new insight into MXene-based absorbers with enhanced ability to absorb electromagnetic wave by incorporating the magnetic components and 2D rGO sheets.
引用
收藏
页数:11
相关论文
共 68 条
[1]   SnS nanoparticles anchored on Ti3C2 nanosheets matrix via electrostatic attraction method as novel anode for lithium ion batteries [J].
Ai, Jinjin ;
Lei, Yike ;
Yang, Shuai ;
Lai, Chunyan ;
Xu, Qunjie .
CHEMICAL ENGINEERING JOURNAL, 2019, 357 :150-158
[2]   Graphene-enabled electrically switchable radar-absorbing surfaces [J].
Balci, Osman ;
Polat, Emre O. ;
Kakenov, Nurbek ;
Kocabas, Coskun .
NATURE COMMUNICATIONS, 2015, 6
[3]   Variable-Temperature Electron Transport and Dipole Polarization Turning Flexible Multifunctional Microsensor beyond Electrical and Optical Energy [J].
Cao, Mao-Sheng ;
Wang, Xi-Xi ;
Zhang, Min ;
Cao, Wen-Qiang ;
Fang, Xiao-Yong ;
Yuan, Jie .
ADVANCED MATERIALS, 2020, 32 (10)
[4]   2D MXenes: Electromagnetic property for microwave absorption and electromagnetic interference shielding [J].
Cao, Mao-Sheng ;
Cai, Yong-Zhu ;
He, Peng ;
Shu, Jin-Cheng ;
Cao, Wen-Qiang ;
Yuan, Jie .
CHEMICAL ENGINEERING JOURNAL, 2019, 359 :1265-1302
[5]   The effects of temperature and frequency on the dielectric properties, electromagnetic interference shielding and microwave-absorption of short carbon fiber/silica composites [J].
Cao, Mao-Sheng ;
Song, Wei-Li ;
Hou, Zhi-Ling ;
Wen, Bo ;
Yuan, Jie .
CARBON, 2010, 48 (03) :788-796
[6]   Thermally Driven Transport and Relaxation Switching Self-Powered Electromagnetic Energy Conversion [J].
Cao, Maosheng ;
Wang, Xixi ;
Cao, Wenqiang ;
Fang, Xiaoyong ;
Wen, Bo ;
Yuan, Jie .
SMALL, 2018, 14 (29)
[7]   2D/2D Heterojunction of Ultrathin MXene/Bi2WO6 Nanosheets for Improved Photocatalytic CO2 Reduction [J].
Cao, Shaowen ;
Shen, Baojia ;
Tong, Tong ;
Fu, Junwei ;
Yu, Jiaguo .
ADVANCED FUNCTIONAL MATERIALS, 2018, 28 (21)
[8]   Bi2WO6/Nb2CTx MXene hybrid nanosheets with enhanced visible-light-driven photocatalytic activity for organic pollutants degradation [J].
Cui, Ce ;
Guo, Ronghui ;
Xiao, Hongyan ;
Ren, Erhui ;
Song, Qingshuang ;
Xiang, Cheng ;
Lai, Xiaoxu ;
Lan, Jianwu ;
Jiang, Shouxiang .
APPLIED SURFACE SCIENCE, 2020, 505
[9]   Flexible and ultrathin electrospun regenerate cellulose nanofibers and d-Ti3C2Tx (MXene) composite film for electromagnetic interference shielding [J].
Cui, Ce ;
Xiang, Cheng ;
Geng, Liang ;
Lai, Xiaoxu ;
Guo, Ronghui ;
Zhang, Yong ;
Xiao, Hongyan ;
Lan, Jianwu ;
Lin, Shaojian ;
Jiang, Shouxiang .
JOURNAL OF ALLOYS AND COMPOUNDS, 2019, 788 :1246-1255
[10]   Facile Synthesis of Fe@Fe3C/C Nanocomposites Derived from Bulrush for Excellent Electromagnetic Wave-Absorbing Properties [J].
Fan, Guohua ;
Jiang, Yuliang ;
Xin, Jiahao ;
Zhang, Zidong ;
Fu, Xueyan ;
Xie, Peitao ;
Cheng, Chuanbing ;
Liu, Yao ;
Qu, Yunpeng ;
Sun, Kai ;
Fan, Runhua .
ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2019, 7 (23) :18765-+