Facile Construction of Bi2Sn2O7/g-C3N4 Heterojunction with Enhanced Photocatalytic Degradation of Norfloxacin

被引:20
作者
Zhu, Zhengru [1 ]
Xia, Haiwen [1 ]
Li, Hong [2 ]
Han, Songlin [1 ]
机构
[1] Liaoning Normal Univ, Sch Geog, Dalian 116029, Peoples R China
[2] Dalian Naval Acad, Dept Basic, Dalian 116018, Peoples R China
关键词
Bi2Sn2O7; g-C3N4; heterojunction; photocatalyst; norfloxacin; water pollution control; NANOCOMPOSITE; TETRACYCLINE; PERFORMANCE; G-C3N4; NANOPARTICLES; FABRICATION; NANOSHEETS; COMPOSITE;
D O I
10.3390/inorganics10090131
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
To mitigate antibiotic residues in the water environment, Bi2Sn2O7/g-C3N4 (BSCN) heterojunction was fabricated by a facile ultrasound-assisted hydrothermal method. The microstructure, morphology, and optical properties of Bi2Sn2O7/g-C3N4 heterojunction was studied by XRD, FTIR, XPS, SEM, TEM, UV-Vis DRS, and PL. The degradation rate of 20 mg/L norfloxacin (NOR) under visible light for 3 h was adopted as one of the indexes to evaluate the photocatalytic performance of Bi2Sn2O7/g-C3N4 heterojunction. Embellished with 20% Bi2Sn2O7 (BSO), the Bi2Sn2O7/g-C3N4 heterojunction decomposed 94% NOR in the experimental solution, which was 2.35 and 3.03 times as much as pristine g-C3N4 and bare Bi2Sn2O7, respectively. In addition, the Bi2Sn2O7/g-C3N4 heterojunction still eliminated 89% of NOR after five cycles, portending outstanding stability and cyclability of photocatalytic activity. A possible photocatalytic mechanism of Bi2Sn2O7/g-C3N4 heterojunction for NOR degradation is proposed.
引用
收藏
页数:13
相关论文
共 60 条
[41]   Br-doping of g-C3N4 towards enhanced photocatalytic performance in Cr(VI) reduction [J].
Wang, Mian ;
Zeng, Yubin ;
Dong, Guohui ;
Wang, Chuanyi .
CHINESE JOURNAL OF CATALYSIS, 2020, 41 (10) :1498-1510
[42]   Synthesis of redox-mediator-free direct Z-scheme AgI/WO3 nanocomposite photocatalysts for the degradation of tetracycline with enhanced photocatalytic activity [J].
Wang, Tianyong ;
Quan, Wei ;
Jiang, Deli ;
Chen, Linlin ;
Li, Di ;
Meng, Suci ;
Chen, Min .
CHEMICAL ENGINEERING JOURNAL, 2016, 300 :280-290
[43]   Photocatalytic properties of a new Z-scheme system BaTiO3/In2S3 with a core-shell structure [J].
Wei, Kaili ;
Wang, Baolai ;
Hu, Jiamin ;
Chen, Fuming ;
Hao, Qing ;
He, Guannan ;
Wang, Yinzhen ;
Li, Wei ;
Liu, Junming ;
He, Qinyu .
RSC ADVANCES, 2019, 9 (20) :11377-11384
[44]   Improved visible-light photocatalysis of nano-Bi2Sn2O7 with dispersed s-bands [J].
Wu, Jianjun ;
Huang, Fuqiang ;
Lue, Xujie ;
Chen, Ping ;
Wan, Dongyun ;
Xu, Fangfang .
JOURNAL OF MATERIALS CHEMISTRY, 2011, 21 (11) :3872-3876
[45]   In2O3/Bi2Sn2O7 heterostructured nanoparticles with enhanced photocatalytic activity [J].
Xing, Yonglei ;
Que, Wenxiu ;
Yin, Xingtian ;
He, Zuoli ;
Liu, Xiaobin ;
Yang, Yawei ;
Shao, Jinyou ;
Kong, Ling Bing .
APPLIED SURFACE SCIENCE, 2016, 387 :36-44
[46]   Reduced graphene oxide/Bi4O5Br2 nanocomposite with synergetic effects on improving adsorption and photocatalytic activity for the degradation of antibiotics [J].
Xu, Mengwen ;
Wang, Yanying ;
Ha, Enna ;
Zhang, Huijuan ;
Li, Chunya .
CHEMOSPHERE, 2021, 265
[47]   Novel heterostructured Bi2S3/Bi2Sn2O7 with highly visible light photocatalytic activity for the removal of rhodamine B [J].
Xu, Weicheng ;
Fang, Jianzhang ;
Chen, Yunfang ;
Lu, Shaoyou ;
Zhou, Guangying ;
Zhu, Ximiao ;
Fang, Zhanqiang .
MATERIALS CHEMISTRY AND PHYSICS, 2015, 154 :30-37
[48]   Novel visible-light-induced BiOCl/g-C3N4 photocatalyst for efficient degradation of metronidazole [J].
Xu, Yao ;
Li, Zhuozhe ;
Fang, Fang ;
Yifeng, E. ;
Zhao, Guizhi .
INORGANIC CHEMISTRY COMMUNICATIONS, 2021, 132
[49]   Controlled growth of "cookie-like" ZnIn2S4 nanoparticles on g-C3N4 for enhanced visible light photocatalytic activity [J].
Xu, Yao ;
E, Yifeng ;
Wang, Guannan .
INORGANIC CHEMISTRY COMMUNICATIONS, 2019, 108
[50]   Dual Z-Scheme CuO-ZnO@Graphitic Carbon Nitride Ternary Nanocomposite with Improved Visible Light-Induced Catalytic Activity for Ultrasound-Assisted Photocatalytic Desulfurization [J].
Yaghoot-Nezhad, Ali ;
Moradi, Mohsen ;
Rostami, Mohammad ;
Danaee, Iman ;
Khosravi-Nikou, Mohammad Reza .
ENERGY & FUELS, 2020, 34 (11) :13588-13605