Single-molecule optoelectronics

被引：198

作者：

Lee, TH ^{[1
]}

Gonzalez, JI ^{[1
]}

Zheng, J ^{[1
]}

Dickson, RM ^{[1
]}

机构：

[1] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA

来源：

ACCOUNTS OF CHEMICAL RESEARCH | 2005年 / 38卷 / 07期

关键词：

D O I：

10.1021/ar040146t

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

With discrete states, several-atom Ag,, nanoclusters exhibit molecule-like behavior with strong visible fluorescence and robust optical properties. This new class of single-molecule fluorophores has been created and electrically contacted in thin films to produce the first electroluminescent single molecules. A direct reporter of nanoscale charge injection and transport through discrete energy levels, bright Ag,, electroluminescence has been harnessed to create single-molecule light-emitting diodes (LEDs) and optoelectronic logic gates and even to demonstrate full addition operations. These experiments utilizing the small size and quantum behavior of individual Ag nanoclusters usher in the new field of single-molecule optoelectronics.

引用

页码：534 / 541

页数：8

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