Enhanced sputtering from nanoparticles and thin films:: Size effects

被引:53
作者
Jarvi, T. T. [1 ]
Pakarinen, J. A. [1 ]
Kuronen, A. [1 ]
Nordlund, K. [1 ]
机构
[1] Univ Helsinki, Dept Phys, FI-00014 Helsinki, Finland
关键词
D O I
10.1209/0295-5075/82/26002
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Sputtering of gold nanoparticles and nanometer-thin films under 25 keV gallium-ion bombardment is shown, using molecular-dynamics simulations, to be significantly enhanced compared to bulk. The highest yield, about three times that of bulk gold, occurs for particles of about 8nm in diameter. For thin films, the maximal yield is obtained for roughly 3 nm thick films. A model based on the work of Sigmund is presented to explain the size-dependence. Copyright (c) EPLA, 2008.
引用
收藏
页数:4
相关论文
共 17 条
[1]   Metal-assisted secondary ion mass spectrometry: Influence of Ag and Au deposition on molecular ion yields [J].
Adriaensen, L ;
Vangaever, F ;
Gijbels, R .
ANALYTICAL CHEMISTRY, 2004, 76 (22) :6777-6785
[2]  
Arfken G.B., 2005, Mathematical Methods for Physicists, V6th edn
[3]   THEORY OF RIPPLE TOPOGRAPHY INDUCED BY ION-BOMBARDMENT [J].
BRADLEY, RM ;
HARPER, JME .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A-VACUUM SURFACES AND FILMS, 1988, 6 (04) :2390-2395
[4]   Ion beam induced destabilization of icosahedral structures in gas phase prepared FePt nanoparticles -: art. no. 10N112 [J].
Dmitrieva, O ;
Rellinghaus, B ;
Kästner, J ;
Liedke, MO ;
Fassbender, J .
JOURNAL OF APPLIED PHYSICS, 2005, 97 (10)
[5]   Structural modification of a multiply twinned nanoparticle by ion irradiation:: A molecular dynamics study [J].
Jarvi, T. T. ;
Kuronen, A. ;
Nordlund, K. ;
Albe, K. .
JOURNAL OF APPLIED PHYSICS, 2007, 102 (12)
[6]  
JARVI TT, UNPUB
[7]   Sputtering from spherical Au clusters by energetic atom bombardment [J].
Kissel, R ;
Urbassek, HM .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 2001, 180 :293-298
[8]   Metal nanoparticle deposition for TOF-SIMS signal enhancement of polymers [J].
Marcus, A ;
Winograd, N .
ANALYTICAL CHEMISTRY, 2006, 78 (01) :141-148
[9]  
POHL D, UNPUB
[10]   THEORY OF CHEMICAL BONDING BASED ON THE ATOM-HOMOGENEOUS ELECTRON-GAS SYSTEM [J].
RAEKER, TJ ;
DEPRISTO, AE .
INTERNATIONAL REVIEWS IN PHYSICAL CHEMISTRY, 1991, 10 (01) :1-54