Heterogeneous photocatalytic oxidation of organics for air purification by near UV irradiated titanium dioxide

被引:100
作者
Hager, S [1 ]
Bauer, R [1 ]
机构
[1] Vienna Tech Univ, Inst Phys Chem, A-1060 Vienna, Austria
关键词
D O I
10.1016/S0045-6535(98)00375-0
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The photocatalytic degradation of high concentrations of various organic pollutants (acetone, 2-propanol and toluene) in dry and humid air streams was carried out using a specially designed photoreactor based on the UV-TIO, principle. The influence of several parameters which control the destruction efficiency (flow rate, initial contaminant and water vapour concentration, temperature and light intensity) has been studied. The conversion was maximal at room temperature, low flow rates and low initial contaminant concentrations. The presence of water in the inlet stream strongly affected the performance of the catalyst. The primary oxidation product of 2-propanol was acetone.
引用
收藏
页码:1549 / 1559
页数:11
相关论文
共 33 条
[1]   SELECTIVITY CONTROL DURING THE PHOTOASSISTED OXIDATION OF 1-BUTANOL ON TITANIUM-DIOXIDE [J].
BLAKE, NR ;
GRIFFIN, GL .
JOURNAL OF PHYSICAL CHEMISTRY, 1988, 92 (20) :5697-5701
[2]   FLUIDIZED-BED PHOTOCATALYTIC OXIDATION OF TRICHLOROETHYLENE IN CONTAMINATED AIRSTREAMS [J].
DIBBLE, LA ;
RAUPP, GB .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1992, 26 (03) :492-495
[3]   KINETICS OF THE GAS-SOLID HETEROGENEOUS PHOTOCATALYTIC OXIDATION OF TRICHLOROETHYLENE BY NEAR UV ILLUMINATED TITANIUM-DIOXIDE [J].
DIBBLE, LA ;
RAUPP, GB .
CATALYSIS LETTERS, 1990, 4 (4-6) :345-354
[4]  
ELAKABI H, 1993, PHOTOCATALYTIC PURIF, pCH7
[5]   THE GAS-PHASE PHOTOCATALYTIC MINERALIZATION OF BENZENE ON POROUS TITANIA-BASED CATALYSTS [J].
FU, XZ ;
ZELTNER, WA ;
ANDERSON, MA .
APPLIED CATALYSIS B-ENVIRONMENTAL, 1995, 6 (03) :209-224
[6]   Effects of reaction temperature and water vapor content on the heterogeneous photocatalytic oxidation of ethylene [J].
Fu, XZ ;
Clark, LA ;
Zeltner, WA ;
Anderson, MA .
JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY, 1996, 97 (03) :181-186
[7]   HETEROGENEOUS PHOTOCATALYSIS - AN EMERGING DISCIPLINE INVOLVING MULTIPHASE SYSTEMS [J].
HERRMANN, JM .
CATALYSIS TODAY, 1995, 24 (1-2) :157-164
[8]   ENVIRONMENTAL APPLICATIONS OF SEMICONDUCTOR PHOTOCATALYSIS [J].
HOFFMANN, MR ;
MARTIN, ST ;
CHOI, WY ;
BAHNEMANN, DW .
CHEMICAL REVIEWS, 1995, 95 (01) :69-96
[9]   NEW REACTOR DESIGN FOR PHOTOCATALYTIC WASTE-WATER TREATMENT WITH TIO2 IMMOBILIZED ON FUSED-SILICA GLASS-FIBERS - PHOTOMINERALIZATION OF 4-CHLOROPHENOL [J].
HOFSTADLER, K ;
BAUER, R ;
NOVALIC, S ;
HEISLER, G .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1994, 28 (04) :670-674
[10]  
HOFSTADLER K, 1994, THESIS VIENNA U TECH