Fast-Response Metal-Semiconductor-Metal Junction Ultraviolet Photodetector Based on ZnS:Mn Nanorod Networks via a Cost-Effective Method

被引:14
作者
Saeed, Sara [1 ,2 ]
Dai, Rucheng [3 ]
Janjua, Raheel Ahmed [3 ,4 ]
Huang, Da [1 ]
Wang, He [1 ]
Wang, Zhongping [3 ]
Ding, Zejun [1 ,2 ]
Zhang, Zengming [1 ,2 ,3 ]
机构
[1] Univ Sci & Technol China, Dept Phys, Hefei 230026, Anhui, Peoples R China
[2] Univ Sci & Technol China, CAS Key Lab Strong Coupled Quantum Matter Phys, Hefei 230026, Anhui, Peoples R China
[3] Univ Sci & Technol China, Ctr Phys Expt, Hefei 230026, Peoples R China
[4] Zhejiang Univ, Coll Opt Sci & Engn, Natl Engn Res Ctr Opt Instruments, Hangzhou 310058, Peoples R China
基金
中国国家自然科学基金;
关键词
EMISSION BANDS; NANOWIRES; TEMPERATURE; LUMINESCENCE; PERFORMANCE; TRANSITION; BEHAVIOR;
D O I
10.1021/acsomega.1c04981
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In this work, Mn2+-doped ZnS nanorods were synthesized by a facile hydrothermal method. The morphology, structure, and composition of the as-prepared samples were investigated. The temperature-dependent photoluminescence of ZnS:Mn nanorods was analyzed, and the corresponding activation energies were calculated by using a simple two-step rate equation. Mn2+-related orange emission (T-4(1) -> (6)A(1)) demonstrates high stability and is comparatively less affected by the temperature variations than the defect-related emission. A metal-semiconductor-metal junction ultraviolet photodetector based on the nanorod networks has been fabricated by a cost-effective method. The device exhibits visible blindness, superior ultraviolet photodetection with a responsivity of 1.62 A/W, and significantly fast photodetection response with the rise and decay times of 12 and 25 ms, respectively.
引用
收藏
页码:32930 / 32937
页数:8
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