Propulsion and controlled steering of magnetic nanohelices

被引:15
作者
Alcanzare, Maria Michiko [1 ]
Karttunen, Mikko [2 ]
Ala-Nissila, Tapio [3 ,4 ,5 ,6 ]
机构
[1] Aalto Univ, Dept Appl Phys, HYBER CoE, FI-00076 Aalto, Finland
[2] Western Univ, Dept Chem & Appl Math, 1151 Richmond St, London, ON N6A 5B7, Canada
[3] Aalto Univ, Dept Appl Phys, QTF CoE, FI-00076 Aalto, Finland
[4] Loughborough Univ, Ctr Interdisciplinary Math Modelling, Loughborough LE11 3TU, Leics, England
[5] Loughborough Univ, Dept Math Sci, Loughborough LE11 3TU, Leics, England
[6] Loughborough Univ, Dept Phys, Loughborough LE11 3TU, Leics, England
基金
加拿大自然科学与工程研究理事会; 芬兰科学院;
关键词
CATALYTIC NANOMOTORS; AUTONOMOUS MOVEMENT; PARTICLES; DRIVEN; NANOPARTICLES; DELIVERY; MOTORS; MOTION;
D O I
10.1039/c8sm00037a
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Externally controlled motion of micro and nanomotors in a fluid environment constitutes a promising tool in biosensing, targeted delivery and environmental remediation. In particular, recent experiments have demonstrated that fuel-free propulsion can be achieved through the application of external magnetic fields on magnetic helically shaped structures. The magnetic interaction between helices and the rotating field induces a torque that rotates and propels them via the coupled rotational-translational motion. Recent works have shown that there exist certain optimal geometries of helical shapes for propulsion. However, experiments show that controlled motion remains a challenge at the nanoscale due to Brownian motion that interferes with the deterministic motion and makes it difficult to achieve controlled steering. In the present work we employ quantitatively accurate simulation methodology to design a setup for which magnetic nanohelices of 30 nm in radius and 180 nm in length (corresponding to previously determined optimal length to radius ratio of 6), with and without cargo, can be accurately propelled and steered in the presence of thermal fluctuations. In particular, we demonstrate fast transport of such nanomotors and devise protocols in manipulating external fields to achieve directionally controlled steering at biologically relevant temperatures.
引用
收藏
页码:1684 / 1691
页数:8
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