Theoretical analysis of X-ray magnetic circular dichroism at the Yb L2, 3 absorption edges of YbInCu4 in high magnetic fields around the field-induced valence transition

被引:12
作者
Kotani, A. [1 ,2 ]
机构
[1] Photon Factory, Inst Mat Struct Sci, Tsukuba, Ibaraki 3050801, Japan
[2] RIKEN SPring 8 Ctr, Mikazuki, Hyogo 6795148, Japan
基金
日本学术振兴会;
关键词
CE; SPECTRA; MODEL;
D O I
10.1140/epjb/e2011-20577-y
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
High-magnetic-field X-ray absorption spectra (XAS) and its X-ray magnetic circular dichroism (XMCD) at the Yb L-2,L- 3 edges of YbInCu4 are calculated around the field-induced valence transition at about 30 T. The calculations are made by using a new theoretical framework with an extended single impurity Anderson model (SIAM) developed recently by the present author. Two parameters in SIAM, the 4f level and the hybridization strength, are taken as different values in low-and high-magnetic-field phases of the field-induced valence transition. The calculated results are compared with recent experimental data measured by Matsuda et al. by utilizing a miniature pulsed magnet up to 40 T. The field-dependence of the calculated XMCD spectra is explained in detail on the basis of the field-dependence of the Yb 4f wavefunctions in the ground state. Some possibilities are discussed on the negative XMCD signal observed experimentally at the L-2 edge.
引用
收藏
页数:12
相关论文
共 35 条
[11]   Low-temperature properties of the Ce(Pd1-xNix)3 system [J].
Kappler, JP ;
Herr, A ;
Schmerber, G ;
Derory, A ;
Parlebas, JC ;
Jaouen, N ;
Wilhelm, F ;
Rogalev, A .
EUROPEAN PHYSICAL JOURNAL B, 2004, 37 (02) :163-167
[12]   Crystal field effect on X-ray magnetic circular dichroism spectra at the L2,3 absorption edges of mixed-valence Ce and Yb compounds in high magnetic fields [J].
Kotani, A. .
EUROPEAN PHYSICAL JOURNAL B, 2011, 81 (01) :49-62
[13]   THEORY OF MULTIPLET STRUCTURE IN 4D CORE PHOTOABSORPTION SPECTRA OF CEO2 [J].
KOTANI, A ;
OGASAWARA, H ;
OKADA, K ;
THOLE, BT ;
SAWATZKY, GA .
PHYSICAL REVIEW B, 1989, 40 (01) :65-73
[14]   Theory of high-magnetic-field XAS and XMCD spectra at the Yb L and M edges around the field-induced valence transition of YbInCu4 [J].
Kotani, A. .
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 2010, 181 (2-3) :168-172
[15]   Effect of a finite conduction-band width on XMCD spectra at the L2,3 absorption edges of mixed-valence Ce and Yb compounds in high magnetic fields [J].
Kotani, A. .
EUROPEAN PHYSICAL JOURNAL B, 2009, 72 (03) :375-384
[16]  
Kotani A, 2008, PHYS REV B, V78, DOI 10.1103/PhysRevB.78.195115
[17]   Theory of XMCD spectra at the L2,3 absorption edges of mixed valence Ce and Yb compounds in high magnetic fields [J].
Kotani, A. .
EUROPEAN PHYSICAL JOURNAL-SPECIAL TOPICS, 2009, 169 :191-197
[18]   Theoretical and experimental study of high-magnetic-field XMCD spectra at the L2,3 absorption edges of mixed-valence rare-earth compounds [J].
Kotani, Akio ;
Matsuda, Yasuhiro H. ;
Nojiri, Hiroyuki .
14TH INTERNATIONAL CONFERENCE ON X-RAY ABSORPTION FINE STRUCTURE (XAFS14), PROCEEDINGS, 2009, 190
[19]   Theory of X-ray magnetic circular dichroism at L2,3 absorption edges of Ce compounds [J].
Kotani, Akio .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2008, 77 (01)
[20]   RAISING OF ANGULAR MOMENTUM DEGENERACY OF F-ELECTRON TERMS BY CUBIC CRYSTAL FIELDS [J].
LEA, KR ;
LEASK, MJM ;
WOLF, WP .
JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS, 1962, 23 (OCT) :1381-&