Effect of air flow on liquid water transport through a hydrophobic gas diffusion layer of a polymer electrolyte membrane fuel cell

被引:33
作者
Suresh, P. V. [1 ]
Jayanti, S. [1 ]
机构
[1] Indian Inst Technol, Dept Chem Engn, Madras 600036, Tamil Nadu, India
关键词
Gas diffusion layer; Hydrophobicity; Water management; Two-phase flow; Polymer electrolyte membrane fuel cells; Cross-flow; CROSS-FLOW; DYNAMICS; PERFORMANCE; BEHAVIOR; VISUALIZATION; MICROSCALE; CHALLENGES; MANAGEMENT; DROPLETS; REMOVAL;
D O I
10.1016/j.ijhydene.2010.04.052
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The transport of liquid water through an idealized 2-D reconstructed gas diffusion layer (GDL) of a polymer electrolyte membrane (PEM) fuel cell is computed subject to hydrophobic boundary condition at the fibre fluid interface. The effect of air flow, as would occur in parallel/serpentine/interdigitated type of flow fields, on the liquid water transport through the GDL, ejection into the channel in the form of water droplets and subsequent removal of the droplets has been simulated. Results show that typically water flow through the fibrous GDL occurs through a fingering and channelling type of mechanism. The presence of cross-flow of air has an effect both on the path created within the GDL and on the ejection of water into the channel in the form of droplets. A faster rate of liquid water evacuation through the GDL (i.e., more frequent ejection of water droplets) as well as less flooding of the void space results from the presence of cross-flow. These results agree qualitatively with experimental observations reported in the literature. (C) 2010 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:6872 / 6886
页数:15
相关论文
共 36 条
[1]   Investigation of water droplet kinetics and optimization of channel geometry for PEM fuel cell cathodes [J].
Akhtar, Nawaz ;
Qureshi, Arshad ;
Scholta, Joachim ;
Hartnig, Christoph ;
Messerschmidt, Matthias ;
Lehnert, Weyner .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2009, 34 (07) :3104-3111
[2]   Liquid water visualization in PEM fuel cells: A review [J].
Bazylak, A. .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2009, 34 (09) :3845-3857
[3]   Dynamic water transport and droplet emergence in PEMFC gas diffusion layers [J].
Bazylak, Aimy ;
Sinton, David ;
Djilali, Ned .
JOURNAL OF POWER SOURCES, 2008, 176 (01) :240-246
[4]   A CONTINUUM METHOD FOR MODELING SURFACE-TENSION [J].
BRACKBILL, JU ;
KOTHE, DB ;
ZEMACH, C .
JOURNAL OF COMPUTATIONAL PHYSICS, 1992, 100 (02) :335-354
[5]   Effects of hydrophilic/hydrophobic properties on the water behavior in the micro-channels of a proton exchange membrane fuel cell [J].
Cai, Y. H. ;
Hu, J. ;
Ma, H. P. ;
Yi, B. L. ;
Zhang, H. M. .
JOURNAL OF POWER SOURCES, 2006, 161 (02) :843-848
[6]   Transport phenomena in fuel cells: from microscale to macroscale [J].
Djilali, N. ;
Sui, P. C. .
INTERNATIONAL JOURNAL OF COMPUTATIONAL FLUID DYNAMICS, 2008, 22 (1-2) :115-133
[7]   Computational modelling of polymer electrolyte membrane (PEM) fuel cells: Challenges and opportunities [J].
Djilali, N. .
ENERGY, 2007, 32 (04) :269-280
[8]   Multiphase flow model to study channel flow dynamics of PEM fuel cells: deformation and detachment of water droplets [J].
Golpaygan, Amirreza ;
Ashgriz, Nasser .
INTERNATIONAL JOURNAL OF COMPUTATIONAL FLUID DYNAMICS, 2008, 22 (1-2) :85-95
[9]   In-plane and through-plane gas permeability of carbon fiber electrode backing layers [J].
Gostick, Jeff T. ;
Fowler, Michael W. ;
Pritzker, Mark D. ;
Ioannidis, Marios A. ;
Behra, Leya M. .
JOURNAL OF POWER SOURCES, 2006, 162 (01) :228-238
[10]   VOLUME OF FLUID (VOF) METHOD FOR THE DYNAMICS OF FREE BOUNDARIES [J].
HIRT, CW ;
NICHOLS, BD .
JOURNAL OF COMPUTATIONAL PHYSICS, 1981, 39 (01) :201-225