Suppression of dewetting phenomena during excimer laser melting of thin metal films on SiO2

被引:15
作者
Kline, JE [1 ]
Leonard, JP [1 ]
机构
[1] Univ Pittsburgh, Dept Mat Sci & Engn, Pittsburgh, PA 15261 USA
关键词
laser irradiation; gold; nickel; wetting;
D O I
10.1016/j.tsf.2005.04.037
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Pulsed. excimer laser irradiation has been used to fully melt 200 nm films of elemental An and Ni on SiO2 substrates. With the use of a capping layer Of SiO2 and line irradiation via projection optics, the typical liquid-phase dewetting processes associated with these metals on SiO2 has been suppressed. In a series of experiments varying line widths and fluence, a process region is revealed immediately above the complete melting threshold for which the films remain continuous and smooth after melting and resolidification. Simple energetic arguments for mechanisms leading to initiation of dewetting support these observations, and a gas-mediated model is proposed to describe the process conditions that are necessary for the suppression of dewetting. (c) 2005 Elsevier B.V. All rights reserved.
引用
收藏
页码:306 / 313
页数:8
相关论文
共 42 条
[1]   Thermocapillary flow and rupture in films of molten metal on a substrate [J].
Ajaev, VS ;
Willis, DA .
PHYSICS OF FLUIDS, 2003, 15 (10) :3144-3150
[2]   METAL-FILM REMOVAL AND PATTERNING USING A XECL LASER [J].
ANDREW, JE ;
DYER, PE ;
GREENOUGH, RD ;
KEY, PH .
APPLIED PHYSICS LETTERS, 1983, 43 (11) :1076-1078
[3]  
[Anonymous], 1993, RAPID SOLIDIFICATION
[4]   Parameter-free test of alloy dendrite-growth theory [J].
Arnold, CB ;
Aziz, MJ ;
Schwarz, M ;
Herlach, DM .
PHYSICAL REVIEW B, 1999, 59 (01) :334-343
[5]  
ATWATER HA, 1980, MATER RES SOC S P, V157, P369
[6]   The solidification velocity of pure nickel [J].
Bassler, BT ;
Hofmeister, WH ;
Bayuzick, RJ .
MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING, 2003, 342 (1-2) :80-92
[7]   LASER-SURFACE PROCESSING OF METALS AND CERAMICS FOR INDUSTRIAL APPLICATIONS [J].
BERGMANN, HW ;
SCHUTTE, K ;
SCHUBERT, E ;
EMMEL, A .
APPLIED SURFACE SCIENCE, 1995, 86 (1-4) :259-265
[8]   Dewetting modes of thin metallic films: Nucleation of holes and spinodal dewetting [J].
Bischof, J ;
Scherer, D ;
Herminghaus, S ;
Leiderer, P .
PHYSICAL REVIEW LETTERS, 1996, 77 (08) :1536-1539
[9]   LASER-INDUCED MORPHOLOGY CHANGES IN THIN COPPER-FILMS [J].
BLOCH, J ;
ZEIRI, Y .
JOURNAL OF APPLIED PHYSICS, 1987, 61 (07) :2637-2644
[10]   Nanosecond time-resolved reflectivity determination of the melting of metals upon pulsed laser annealing [J].
Boneberg, J ;
Bischof, J ;
Leiderer, P .
OPTICS COMMUNICATIONS, 2000, 174 (1-4) :145-149