Metastable magnetic phases induced by rotation of α-Dy2S3 single crystal in magnetic field

被引:3
作者
Ebisu, Shuji [1 ]
Fuji, Koichiro [1 ]
Guo, Qing [1 ]
Miyazaki, Masanori [1 ]
机构
[1] Muroran Inst Technol, Div Appl Sci, 27-1 Mizumoto Cho, Muroran, Hokkaido 0508585, Japan
基金
日本学术振兴会;
关键词
Rare earth sesquisulfide; Metastable magnetic phase; Single crystal rotation; Magnetization enhancement; Easy magnetization axis switch; RARE-EARTH SESQUISULFIDES; ALPHA-GD2S3; TRANSITION; DIFFRACTION; DYCU2;
D O I
10.1016/j.jmmm.2017.08.018
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Metastable magnetic phases in alpha-Dy2S3 induced by rotation of the single crystal in a magnetic field have been investigated. The compound alpha-Dy2S3 possesses an orthorhombic crystal structure having two crystallographically inequivalent Dy sites and shows successive antiferromagnetic transitions at T-N1 = 11.4 K and T-N2 = 6.4 K associated with various steep responses in physical properties. Anomalous enhancement of the alpha-axis magnetization from 5.4 to 8.4 mu(B)/Dy-atom has been found after a certain process of rotating the single crystal at 6 K around the b-axis in the magnetic field of 7 T perpendicular to the b-axis. This magnetic phase induced by rotating the single crystal has been considered as the same phase induced by cooling in the strong magnetic field of 18 T, which had been found in our previous work. Moreover, a certain process that combines rotating with cooling of the single crystal in the magnetic field gives rise to exchange of the features of the magnetization curves for the a-and c-direction. Consequently, the easy magnetization axis in the ac-plane switches to the c-axis from the a-axis. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:140 / 145
页数:6
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