Yield, variance and spatial distribution of electron-hole pairs in CsI

被引:19
作者
Gao, F. [1 ]
Xie, Y. [1 ]
Kerisit, S. [1 ]
Campbell, L. W. [1 ]
Weber, W. J. [2 ,3 ]
机构
[1] Pacific NW Natl Lab, Richland, WA 99352 USA
[2] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA
[3] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA
关键词
Monte Carlo simulation; Intrinsics properties; Spatial distribution; Electron-hole pairs; CsI; NON-PROPORTIONALITY; CROSS-SECTIONS; SCATTERING; ENERGIES; SIMULATION; POSITRONS;
D O I
10.1016/j.nima.2010.08.063
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
A Monte Carlo (MC) method previously developed has been applied to simulate the interaction of photons, with energies ranging from 50 eV to similar to 1 MeV, with CsI and the subsequent electron cascades. The MC model has been employed to compute nano-scale spatial distributions of electron-hole pairs and important intrinsic properties, including W, the mean energy per electron-hole pair, and the Fano factor, F. W exhibits discontinuities at the shell edges that follow the photoionization cross-sections and decreases with increase in photon energy (from similar to 19 to 15 eV), with an asymptotic value of 15.2 eV at high energy. This decrease may contribute to the initial rise in relative light yield with incident energy observed experimentally for CsI, thus suggesting that nonlinearity may be associated with intrinsic properties of the material at low energies. F is calculated to increase with increase in energy and has an asymptotic value of 0.28. A significant number of electron-hole pairs is produced through the different ionization channels of core shells and the corresponding relaxation processes, which may explain why F is larger for CsI than for Si or Ge. Finally, the calculated spatial distributions show that the electron-hole pairs are primarily distributed along fast electron tracks. These spatial distributions constitute important input for large-scale simulations of electron-hole pair transport. (C) 2010 Elsevier B.V. All rights reserved.
引用
收藏
页码:564 / 567
页数:4
相关论文
共 25 条
[1]   Mixed simulation of the multiple elastic scattering of electrons and positrons using partial-wave differential cross-sections [J].
Benedito, E ;
Fernández-Varea, JM ;
Salvat, F .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 2001, 174 (1-2) :91-110
[2]  
BERGER MJ, 1987, NBSIR873597
[3]   The role of different linear and non-linear channels of relaxation in scintillator non-proportionality [J].
Bizarri, G. ;
Moses, W. W. ;
Singh, J. ;
Vasil'ev, A. N. ;
Williams, R. T. .
JOURNAL OF LUMINESCENCE, 2009, 129 (12) :1790-1793
[4]   Simple model relating recombination rates and non-proportional light yield in scintillators [J].
Bizarri, G. ;
Moses, W. W. ;
Singh, J. ;
Vasil'ev, A. N. ;
Williams, R. T. .
PHYSICA STATUS SOLIDI C - CURRENT TOPICS IN SOLID STATE PHYSICS, VOL 6, NO 1, 2009, 6 (01) :97-+
[5]   An analytical model of nonproportional scintillator light yield in terms of recombination rates [J].
Bizarri, G. ;
Moses, W. W. ;
Singh, J. ;
Vasil'ev, A. N. ;
Williams, R. T. .
JOURNAL OF APPLIED PHYSICS, 2009, 105 (04)
[6]   ELECTRON-ACOUSTIC PHONON-SCATTERING IN SIO2 DETERMINED FROM A PSEUDO-POTENTIAL FOR ENERGIES OF E GREATER-THAN EBZ [J].
BRADFORD, JN ;
WOOLF, S .
JOURNAL OF APPLIED PHYSICS, 1991, 70 (01) :490-492
[7]   CALCULATION OF ELECTRON SHAKE-OFF PROBABILITIES AS RESULT OF X-RAY PHOTOIONIZATION OF RARE-GASES [J].
CARLSON, TA ;
NESTOR, CW .
PHYSICAL REVIEW A, 1973, 8 (06) :2887-2894
[8]  
Cullen D E, 1997, UCRL50400, V6
[9]   Non-proportionality in the scintillation response and the energy resolution obtainable with scintillation crystals [J].
Dorenbos, P ;
deHaas, JTM ;
vanEijk, CWE .
IEEE TRANSACTIONS ON NUCLEAR SCIENCE, 1995, 42 (06) :2190-2202
[10]   Scintillation mechanisms in Ce3+ doped halide scintillators [J].
Dorenbos, P .
PHYSICA STATUS SOLIDI A-APPLIED RESEARCH, 2005, 202 (02) :195-200