Non-negligible emissions of black carbon from non-road construction equipment based on real-world measurements in China

被引:16
作者
Wu, Bobo [1 ,2 ,3 ]
Xuan, Kaijie [1 ]
Shen, Xianbao [1 ,2 ,3 ]
Zhao, Qiangqiang [1 ]
Shi, Yue [1 ]
Kong, Lei [1 ]
Hu, Jinfeng [1 ]
Li, Xin [1 ,2 ,3 ]
Zhang, Hanyu [1 ,2 ,3 ]
Cao, Xinyue [1 ,2 ,3 ]
Hao, Xuewei [1 ,2 ,3 ]
Zhou, Qi [1 ,2 ,3 ]
Yao, Zhiliang [1 ,2 ,3 ]
机构
[1] Beijing Technol & Business Univ, Sch Ecol & Environm, Beijing 100048, Peoples R China
[2] Beijing Technol & Business Univ, State Environm Protect Key Lab Food Chain Pollut, Beijing 100048, Peoples R China
[3] Beijing Technol & Business Univ, Key Lab Cleaner Prod & Integrated Resource Utiliz, Beijing 100048, Peoples R China
基金
北京市自然科学基金; 中国国家自然科学基金;
关键词
Black carbon; Non-road construction equipment; SP-PEMS; Emission characteristic; Emission factors; PARTICULATE MATTER; DIESEL; EXHAUST;
D O I
10.1016/j.scitotenv.2021.151300
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Non-road construction equipment (NRCE) has become a vital contributor to urban air pollutants with the rapid urbanization in China. Black carbon (BC), as a key pollutant emitted from NRCE (mainly diesel-fueled), has attracted considerable concerns due to adverse impacts on climate change, visibility, and human health. How-ever, the understanding of its emissions is still unclear based on limited research results. In this study, we con-ducted real-world measurements on BC emissions from 12 excavators and 9 loaders to characterize the variation and quantify fuel-based emission factors (EFs) by using a synchronous platform based on PEMS (SP-PEMS). We analyzed the impacts of key factors (operation mode, emission standard, and engine rated power) on BC emission comprehensively. High BC emission in working mode may be mainly owing to the increase of fuel consumption and the deterioration of air-fuel ratio. With more stringent emission standards, BC EFs of all tested NRCE present significant decreasing trends. Interestingly, NRCE with high rated power generally exhibits lower BC emissions. Through comparison, we find BC EFs in this study are generally higher than elemental carbon (EC) EFs reported in previous studies, which will lead BC emissions from NRCE to be underestimated while EC EFs are used instead of BC EFs. Furthermore, BC EFs of NRCE with Stage III are significantly higher (1-3 orders of mag-nitude) than those of on-road diesel trucks with the current mainstream emission standards of China IV and China V, which reinforces the urgency and importance of controlling BC emissions from NRCE in China. Finally, we recommend BC EFs of excavators and loaders under different emission standards and operation modes, and which preliminarily fills the gap in localized BC EFs of typical NRCE to relieve the urgent needs for emission inventory calculation. (c) 2021 Elsevier B.V. All rights reserved.
引用
收藏
页数:8
相关论文
共 49 条
[1]   Long-term changes in emissions of nitrogen oxides and particulate matter from on-road gasoline and diesel vehicles [J].
Ban-Weiss, George A. ;
McLaughlin, John P. ;
Harley, Robert A. ;
Lunden, Melissa M. ;
Kirchstetter, Thomas W. ;
Kean, Andrew J. ;
Strawa, Anthony W. ;
Stevenson, Eric D. ;
Kendall, Gary R. .
ATMOSPHERIC ENVIRONMENT, 2008, 42 (02) :220-232
[2]   Bounding the role of black carbon in the climate system: A scientific assessment [J].
Bond, T. C. ;
Doherty, S. J. ;
Fahey, D. W. ;
Forster, P. M. ;
Berntsen, T. ;
DeAngelo, B. J. ;
Flanner, M. G. ;
Ghan, S. ;
Kaercher, B. ;
Koch, D. ;
Kinne, S. ;
Kondo, Y. ;
Quinn, P. K. ;
Sarofim, M. C. ;
Schultz, M. G. ;
Schulz, M. ;
Venkataraman, C. ;
Zhang, H. ;
Zhang, S. ;
Bellouin, N. ;
Guttikunda, S. K. ;
Hopke, P. K. ;
Jacobson, M. Z. ;
Kaiser, J. W. ;
Klimont, Z. ;
Lohmann, U. ;
Schwarz, J. P. ;
Shindell, D. ;
Storelvmo, T. ;
Warren, S. G. ;
Zender, C. S. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2013, 118 (11) :5380-5552
[3]   Light absorption by carbonaceous particles: An investigative review [J].
Bond, TC ;
Bergstrom, RW .
AEROSOL SCIENCE AND TECHNOLOGY, 2006, 40 (01) :27-67
[4]   A technology-based global inventory of black and organic carbon emissions from combustion [J].
Bond, TC ;
Streets, DG ;
Yarber, KF ;
Nelson, SM ;
Woo, JH ;
Klimont, Z .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D14) :D14203
[5]   Evaluations of in-use emission factors from off-road construction equipment [J].
Cao, Tanfeng ;
Durbin, Thomas D. ;
Russell, Robert L. ;
Cocker, David R., III ;
Scora, George ;
Maldonado, Hector ;
Johnson, Kent C. .
ATMOSPHERIC ENVIRONMENT, 2016, 147 :234-245
[6]   Emission characteristics of polycyclic aromatic hydrocarbons and nitro-polycyclic aromatic hydrocarbons from diesel trucks based on on-road measurements [J].
Cao, Xinyue ;
Hao, Xuewei ;
Shen, Xianbao ;
Jiang, Xi ;
Wu, Bobo ;
Yao, Zhiliang .
ATMOSPHERIC ENVIRONMENT, 2017, 148 :190-196
[7]   Review and Outlook of China Non-Road Diesel Mobile Machinery Emission Standards [J].
Cui Huanxing ;
Li Gang ;
Yuan Ying ;
Ji Liang ;
Liu Shunli .
JOHNSON MATTHEY TECHNOLOGY REVIEW, 2020, 64 (01) :76-83
[8]   Measurement of PM and its chemical composition in real-world emissions from non-road and on-road diesel vehicles [J].
Cui, Min ;
Chen, Yingjun ;
Feng, Yanli ;
Li, Cheng ;
Zheng, Junyu ;
Tian, Chongguo ;
Yan, Caiqing ;
Zheng, Mei .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2017, 17 (11) :6779-6795
[9]   Primary particulate emissions and secondary organic aerosol (SOA) formation from idling diesel vehicle exhaust in China [J].
DengWei ;
HuQihou ;
LiuTengyu ;
WangXinming ;
ZhangYanli ;
SongWei ;
SunYele ;
BiXinhui ;
YuJianzhen ;
YangWeigiang ;
HuangXinyu ;
ZhangZhou ;
HuangZhonghui ;
HeQuanfu ;
Mellouki, Abdelwahid ;
George, Christian .
SCIENCE OF THE TOTAL ENVIRONMENT, 2017, 593 :462-469
[10]   Real-world emissions from non-road mobile machinery in London [J].
Desouza, C. D. ;
Marsh, D. J. ;
Beevers, S. D. ;
Molden, N. ;
Green, D. C. .
ATMOSPHERIC ENVIRONMENT, 2020, 223